Calculation of hydrogen and oxygen uptake in fuel rod cladding during severe accidents using the integral diffusion method -- Preliminary design report
Preliminary designs are described for models of hydrogen and oxygen uptake in fuel rod cladding during severe accidents. Calculation of the uptake involves the modeling of seven processes: (1) diffusion of oxygen from the bulk gas into the boundary layer at the external cladding surface, (2) diffusion from the boundary layer into the oxide layer, (3) diffusion from the inner surface of the oxide layer into the metallic part of the cladding, (4) uptake of hydrogen in the event that the cladding oxide layer is dissolved in a steam-starved region, (5) embrittlement of cladding due to hydrogen uptake, (6) cracking of cladding during quenching due to its embrittlement and (7) release of hydrogen from the cladding after cracking of the cladding. An integral diffusion method is described for calculating the diffusion processes in the cladding. Experimental results are presented that show a rapid uptake of hydrogen in the event of dissolution of the oxide layer and a rapid release of hydrogen in the event of cracking of the oxide layer. These experimental results are used as a basis for calculating the rate of hydrogen uptake and the rate of hydrogen release. The uptake of hydrogen is limited to the equilibrium solubility calculated by applying Sievert's law. The uptake of hydrogen is an exothermic reaction that accelerates the heatup of a fuel rod. An embrittlement criteria is described that accounts for hydrogen and oxygen concentration and the extent of oxidation. A design is described for implementing the models for hydrogen and oxygen uptake and cladding embrittlement into the programming framework of the SCDAP/RELAP5 code. A test matrix is described for assessing the impact of the proposed models on the calculated behavior of fuel rods in severe accident conditions. This report is a revision and reissue of the report entitled; ``Preliminary Design Report for Modeling of Hydrogen Uptake in Fuel Rod Cladding During Severe Accidents.''
- Research Organization:
- Idaho National Lab. (INL), Idaho Falls, ID (United States)
- Sponsoring Organization:
- US Department of Energy (US)
- DOE Contract Number:
- AC07-94ID13223
- OSTI ID:
- 751980
- Report Number(s):
- INEEL/EXT-98-00664(Rev.1); TRN: US0000905
- Resource Relation:
- Other Information: PBD: 1 Feb 1999
- Country of Publication:
- United States
- Language:
- English
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Related Subjects
REACTOR ACCIDENTS
FUEL CANS
MATHEMATICAL MODELS
HYDROGEN
ABSORPTION
DIFFUSION
HYDROGEN EMBRITTLEMENT
OXYGEN
CRACK PROPAGATION
DESORPTION
OXIDATION
S CODES
R CODES
CLADDING EMBRITTLEMENT
OXYGEN DIFFUSION
HYDROGEN UPTAKE
OXYGEN UPTAKE
FUEL ROD CLADDING
SEVERE ACCIDENTS
BOUNDARY LAYER
OXIDE LAYER
QUENCHING
INTEGRAL DIFFUSION METHOD
HYDROGEN RELEASE
EQUILIBRIUM SOLUBILITY
SIEVERT'S LAW
SCDAP/RELAP5