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A Vault Model for the Assessment of Used Fuel Disposal in Canada

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Abstract

The environmental assessment of the geological disposal of used nuclear fuel involves the assimilation of experimental results to produce an estimate of the potential impact of a disposal vault on man and the environment. In this paper we briefly outline the assessment methodology and expand upon one aspect of the data assimilation process, namely, the incorporation of research results on the performance of engineered barriers into assessment models.

The model to be discussed represents (i) failure modes for titaniumbased containers, including short-term failures due to undetected manufacturing defects and long-term failures due to uniform and local corrosion; (ii) release of radionuclides from used fuel, including relatively fast release of soluble fission products from gap and grain boundaries and slow, congruent release controlled by the dissolution of the fuel matrix itself; and (iii) mass transport of released radionuclides through the clay-based sealing materials surrounding the waste container, including diffusion, convection and radionuclide storage (sorption or retardation) effects.

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References

  1. K.W. Dormuth, and R.B. Lyon, “The Link between Detailed Process Models and Simplified Models,” Proc. 2nd NEA Workshop on System Performance Assessment for Radioactive Waste Disposal, Paris. October (1985).

    Google Scholar 

  2. N.C. Garisto, “Modelling Aspects in Vault Chemistry,” in Proc. Second Int. Conf. Radioactive Waste Management, pp. 712–714. Canadian Nuclear Society, Toronto, (1986).

  3. W.T. Hancox, “Progress in the Canadian Nuclear Fuel Waste Management Program,” in Proc. Second Int. Conf. on Radioactive Waste Management, pp. 1–9. Canadian Nuclear Society, Toronto, (1986).

  4. D.M. LeNeveu, “Vault Submodel for the Second Interim Assessment of the Canadian Concept for Nuclear Fuel Waste Disposal: Post-Closure Phase,” Atomic Energy of Canada Limited Report, AECL-8383 (1986).

  5. D.M. Le Neveu, Ann. Nucl. Energy 14, 77 (1987).

    Article  CAS  Google Scholar 

  6. D.M. LeNeveu and N.C. Garisto, “Sensitivity Surfaces for the Predictive Assessment of Waste Package Performance,” submitted to the Scientific Basis for Nuclear Waste Management Symposium, Boston (1987).

  7. D.M. LeNeveu, unpublished results.

  8. K. Nuttall, Can. Metal. Quart. 22 403 (1983).

    Article  CAS  Google Scholar 

  9. G. Doubt, “Assessing Reliability and Useful Life of Containers for Disposal of Irradiated Fuel Waste,” Atomic Energy of Canada Limited Report, AECL-8328 (1984).

  10. M.A. Molecke and L. Abrego, “Status of SANDIA HLW Canister/Overpack Program Studies,” Sandia National Laboratories Report, SAND-80-2191C, (1980).

  11. M.A. Molecke, J.A. Ruppen and R. Diegle, Nucl. Tech. 63, 476 (1983).

    Article  CAS  Google Scholar 

  12. N.R. Sorenson and R.B. Diegle, “Corrosion Research of Alloys for Use in Nuclear Waste Disposal Containers,” in The Corrosion Performance of Nuclear Fuel Waste Containers, pp. 31-40, Atomic Energy of Canada Limited Technical Record, TR-340 (1985).

  13. W.G. Mathers, “HOTROCK, A Program for Calculating the Transient Temperature Field from an Underground Nuclear Waste Disposal Vault,” Atomic Energy of Canada Limited Technical Record, TR-336 (1985).

  14. P. McKay and D.B. Mitton, Corrosion NACE 41, 52 (1985).

    Article  CAS  Google Scholar 

  15. C.F. Clarke, D. Hardie and P. McKay, Corrosion Science, 26, 425 (1986).

    Article  CAS  Google Scholar 

  16. K. Shimogori, H. Sato and H. Tomari, J. Japan Inst. Metals 42, 567 (1978).

    Article  CAS  Google Scholar 

  17. M. Kobayshi, Y. Araya, S. Fujiyama, Y. Sunayama and H. Uno, “Study on Crevice Corrosion of Titanium,” in Titanium ‘80 Science and Technology, Proc. 4th Int. Conf. on Titanium, pp. 2613–2622. The Metallurgical Society of AIME, Warrendale, PA (1980).

  18. H. Sato, F. Kamikubo and K. Shimogori, “Effect of Gasket Materials on Crevice Corrosion of Titanium,” in Titanium ‘84, Proc 5th Int. Conf. on Titanium, Munich, FRG, September 10–14, 1984, edited by G. Lutjering, U. Zwicker and V. Bunk (1985).

  19. M.G. Bailey, B.M. Ikeda, D. Cann and D.W. Shoesmith, “Crevice Corrosion of Titanium Grade-2 under Nuclear Waste Disposal Vault Conditions,” to be published in Proc. Int. Conf. Localized Corrosion, Orlando, Florida, June 1–5 (1987).

  20. B.M. Ikeda and C.F. Clarke, “Titanium Corrosion under Canadian Nuclear Fuel Waste Disposal Conditions,” in Proc. Second Int. Conf. on Radioactive Waste Management, pp. 605–610, Canadian Nuclear Society, Toronto (1986).

  21. R.E. Westerman and M.R. Telander, “Hydrogen Absorption and Crevice Corrosion Behaviour of Ti Grade 12 during Exposure to Irradiated Brine at 150°C” in Waste Management ‘87, Volume 2, pp. 463–469. University of Arizona, Tucson (1987).

  22. N.C Garisto, K.B. Harvey, F. Garisto and L.H. Johnson, “Source Term Models for the Assessment of Nuclear Fuel Waste Disposal in Canada,” in Waste Management ‘86, Volume 2, p. 397. University of Arizona, Tucson (1986).

  23. F. Garisto and N.C. Garisto, Nucl. Sci. Eng. 90, 103 (1985).

    Article  CAS  Google Scholar 

  24. N.C Garisto and F. Garisto, Ann. Nucl. Energy 13, 591 (1986).

    Article  CAS  Google Scholar 

  25. F. Garisto, Chem. Eng. Sci. 41, 3219 (1986).

    Article  CAS  Google Scholar 

  26. N.C Garisto, E.R. Vance, S. Stroes-Gascoyne and L.H. Johnson, “Instant Release Fractions for the Assessment of Used Nuclear Fuel Disposal,” in preparation.

  27. M.G. Bailey, L.H. Johnson and D.W. Shoesmith, Corrosion Sci. 25, 233 (1985).

    Article  CAS  Google Scholar 

  28. F. Garisto, unpublished results.

  29. R.J. Lemire, “Effects of High Ionic Strength Groundwaters on Calculated Equilibrium Concentrations in the Uranium-Water System,” Atomic Energy of Canada Limited Report, in preparation.

  30. T.E. Eriksen and A. Jacobsson, “Diffusion in Clay-Experimental Techniques and Theoretical Models,” KBS Report, KBS-84-05 (1984).

  31. K. Skagius and I. Neretnieks, “Diffusion Measurements of Cesium and Strontium in Biotite Gneiss,” KBS Report, KBS-85-15 (1985).

  32. D.A. Lever “Some Notes on Experiments Measuring Diffusion of Sorbed Nuclides through Porous Media,” Harwell Laboratory Report, AERE R.12321 (1986).

  33. B. Torstenfelt “Migration of Fission Products and Actinides in Compacted Bentonite,” KBS Report 86-14 (1986).

  34. S.C.H. Cheung, “Evaluation of the Methodologies for Determining Ionic Diffusion Coefficients in Clays.” To be published in Proc. CSCE Centennial Conf., May 1987, Montreal, Quebec.

  35. R.W. Gillham, M.J.L. Robin and D.J. Dytynyshyn, Can. Geotech. J. 21, 541 (1984).

    Article  CAS  Google Scholar 

  36. R.W. Gillham, H.M. Johnston, M.J.L. Robin and H.D. Sharma, “Diffusion of Radionuclides in Buffer and Backfill Materials,” in Proceedings of the Nineteenth Information Meeting of the Nuclear Fuel Waste Management Program, pp. 448–464. Atomic Energy of Canada Limited Technical Record, TR-350 (1985).

  37. A.M. Liebetrau, M.J. Apted, D.W. Engel, M.K. Altenhofen, C.R. Reid, D.M. Strachan, R.L. Erikson and D.H. Alexander, “AREST: A Probabilistic Source-Term Code for Waste Package Performance Analysis,” in Waste Management ‘87, Volume 2, pp. 535–544. University of Arizona, (1987).

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Garisto, N.C., Leneveu, D.M. A Vault Model for the Assessment of Used Fuel Disposal in Canada. MRS Online Proceedings Library 112, 313–322 (1987). https://doi.org/10.1557/PROC-112-313

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  • DOI: https://doi.org/10.1557/PROC-112-313

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