Self-Diffusiophoresis of Janus Particles in Near-Critical Mixtures

Alois Würger
Phys. Rev. Lett. 115, 188304 – Published 29 October 2015
PDFHTMLExport Citation

Abstract

We theoretically study the self-propulsion of a laser-heated Janus particle in a near-critical water-lutidine mixture, and we relate its velocity vp and squirmer parameter β to the wetting properties of its two hemispheres. For nonionic surface forces, the particle moves the active cap at the front, whereas a charged hydrophilic cap leads to backward motion, in agreement with the experiment. Both vp and β show nonmonotonic dependencies on the heating power, and they may even change sign. The variation of β is expected to strongly affect the collective behavior of dense squirmer systems.

  • Figure
  • Figure
  • Figure
  • Figure
  • Figure
  • Received 16 March 2015

DOI:https://doi.org/10.1103/PhysRevLett.115.188304

© 2015 American Physical Society

Physics Subject Headings (PhySH)

Polymers & Soft Matter

Authors & Affiliations

Alois Würger

  • Laboratoire Ondes et Matière d’Aquitaine, Université de Bordeaux and CNRS, 351 cours de la Libération, 33405 Talence, France

See Also

Self-Propulsion Mechanism of Active Janus Particles in Near-Critical Binary Mixtures

Sela Samin and René van Roij
Phys. Rev. Lett. 115, 188305 (2015)

Article Text (Subscription Required)

Click to Expand

Supplemental Material (Subscription Required)

Click to Expand

References (Subscription Required)

Click to Expand
Issue

Vol. 115, Iss. 18 — 30 October 2015

Reuse & Permissions
Access Options
Author publication services for translation and copyediting assistance advertisement

Authorization Required


×
×

Images

×

Sign up to receive regular email alerts from Physical Review Letters

Log In

Cancel
×

Search


Article Lookup

Paste a citation or DOI

Enter a citation
×