Lattice theory of trapping reactions with mobile species

M. Moreau, G. Oshanin, O. Bénichou, and M. Coppey
Phys. Rev. E 69, 046101 – Published 14 April 2004
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Abstract

We present a stochastic lattice theory describing the kinetic behavior of trapping reactions A+BB, in which both the A and B particles perform an independent stochastic motion on a regular hypercubic lattice. Upon an encounter of an A particle with any of the B particles, A is annihilated with a finite probability; finite reaction rate is taken into account by introducing a set of two-state random variables—“gates,” imposed on each B particle, such that an open (closed) gate corresponds to a reactive (passive) state. We evaluate here a formal expression describing the time evolution of the A particle survival probability, which generalizes our previous results. We prove that for quite a general class of random motion of the species involved in the reaction process, for infinite or finite number of traps, and for any time t, the A particle survival probability is always larger in the case when A stays immobile, than in situations when it moves.

  • Received 24 April 2003

DOI:https://doi.org/10.1103/PhysRevE.69.046101

©2004 American Physical Society

Authors & Affiliations

M. Moreau1, G. Oshanin1, O. Bénichou2, and M. Coppey1

  • 1Laboratoire de Physique Théorique des Liquides, University Pierre et Marie Curie, 75252 Paris Cedex 05, France
  • 2Laboratoire de Physique de la Matière Condensée, Collège de France, 11 place Marcelin Berthelot, 75005, Paris, France

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Vol. 69, Iss. 4 — April 2004

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