Oscillations and negative velocity autocorrelation emerging from a Brownian particle model with hydrodynamic interactions

A. D. Viñales, M. Camuyrano, and G. H. Paissan
Phys. Rev. E 101, 052140 – Published 28 May 2020

Abstract

We study the dynamics of a particle in a fluid from a generalized Langevin equation (GLE) with a frictional exponential memory kernel and hydrodynamic interactions. By using Laplace analysis we obtain the analytical expressions for the velocity autocorrelation function (VACF) and mean square displacement (MSD) of the particle. Our results show that, in the strictly asymptotic time limit, the dynamics of the particle correspond to a particle ruled by a GLE with a Dirac delta friction memory kernel and hydrodynamic interactions. However, at intermediate times the dynamical behavior is qualitatively different due to the presence of a characteristic time in the frictional exponential memory kernel. Remarkably, the VACF exhibits oscillations and negative correlation regimes which are reminiscent of features already observed in pioneering works of molecular dynamics simulations. Moreover, ripples in the MSD appear as an emerging behavior associated with the mentioned regimes.

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  • Received 15 August 2019
  • Revised 1 November 2019
  • Accepted 6 May 2020

DOI:https://doi.org/10.1103/PhysRevE.101.052140

©2020 American Physical Society

Physics Subject Headings (PhySH)

Statistical Physics & ThermodynamicsCondensed Matter, Materials & Applied Physics

Authors & Affiliations

A. D. Viñales1,*, M. Camuyrano1,2, and G. H. Paissan3,4

  • 1Departamento de Física, Facultad de Ingeniería, Universidad de Buenos Aires, Avenida Paseo Colón 850, C1063ACV Buenos Aires, Argentina
  • 2Comisión Nacional de Actividades Espaciales, Avenida Paseo Colón 751, C1063ACH Buenos Aires, Argentina
  • 3CRUB, Universidad Nacional del Comahue, Quintral 1250, 8400 Bariloche, Río Negro, Argentina
  • 4Centro Atómico Bariloche, CNEA/CONICET, Avenida Bustillo Km 9.5, 8400 Bariloche, Río Negro, Argentina

  • *avinales@fi.uba.ar

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Vol. 101, Iss. 5 — May 2020

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