Time-resolved photoemission of correlated electrons driven out of equilibrium

B. Moritz, T. P. Devereaux, and J. K. Freericks
Phys. Rev. B 81, 165112 – Published 21 April 2010

Abstract

We describe the temporal evolution of the time-resolved photoemission response of the spinless Falicov-Kimball model driven out of equilibrium by strong applied fields. The model is one of the few possessing a metal-insulator transition and admitting an exact solution in the time domain. The nonequilibrium dynamics, evaluated using an extension of dynamical mean-field theory, show how the driven system differs from two common viewpoints—a quasiequilibrium system at an elevated effective temperature (the “hot” electron model) or a rapid interaction quench (“melting” of the Mott gap)—due to the rearrangement of electronic states and redistribution of spectral weight. The results demonstrate the inherent trade-off between energy and time resolution accompanying the finite width probe pulses, characteristic of those employed in pump-probe time-domain experiments, which can be used to focus attention on different aspects of the dynamics near the transition.

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  • Received 1 March 2010

DOI:https://doi.org/10.1103/PhysRevB.81.165112

©2010 American Physical Society

Authors & Affiliations

B. Moritz1,2, T. P. Devereaux1,3, and J. K. Freericks4

  • 1Stanford Institute for Materials and Energy Science (SIMES), SLAC National Accelerator Laboratory, Menlo Park, California 94025, USA
  • 2Department of Physics and Astrophysics, University of North Dakota, Grand Forks, North Dakota 58202, USA
  • 3Geballe Laboratory for Advanced Materials, Stanford University, Stanford, California 94305, USA
  • 4Department of Physics, Georgetown University, Washington, DC 20057, USA

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Issue

Vol. 81, Iss. 16 — 15 April 2010

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