Impurity effects in the quantum kagome system ZnCu3(OH)6Cl2

R. Chitra and M. J. Rozenberg
Phys. Rev. B 77, 052407 – Published 27 February 2008

Abstract

Motivated by the recent experiments on the spin half kagome compound ZnCu3(OH)6Cl2, we study a phenomenological model of a frustrated quantum magnet. The model has a spin liquid ground state and is constructed so as to mimic the macroscopically large quasidegeneracies expected in the low-lying energy structure of a kagome system. We use numerical studies of finite size systems to investigate the static as well as the dynamical responses at finite temperatures. The results obtained using our simple model are compatible with a large number of recent experiments including neutron scattering data. Our study suggests that many of the anomalous features observed in experiments have a natural interpretation in terms of spin-12 defects (impurities) coupled to an underlying kagome-type spin liquid.

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  • Received 4 December 2007

DOI:https://doi.org/10.1103/PhysRevB.77.052407

©2008 American Physical Society

Authors & Affiliations

R. Chitra1 and M. J. Rozenberg2,3

  • 1Laboratoire de Physique Theorique de la Matière Condenseé, UMR 7600, Universite de Pierre et Marie Curie, Jussieu, Paris 75005, France
  • 2Laboratoire de Physique des Solides, CNRS-UMR8502, Université de Paris-Sud, Orsay 91405, France
  • 3Departamento de Física, FCEN, Universidad de Buenos Aires, Ciudad Universitaria Pabellón I, 1428 Buenos Aires, Argentina

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Vol. 77, Iss. 5 — 1 February 2008

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