Mott Transition, Compressibility Divergence, and the PT Phase Diagram of Layered Organic Superconductors: An Ultrasonic Investigation

D. Fournier, M. Poirier, M. Castonguay, and K. D. Truong
Phys. Rev. Lett. 90, 127002 – Published 25 March 2003

Abstract

The phase diagram of the organic superconductor κ(BEDTTTF)2Cu[N(CN)2]Cl has been investigated by ultrasonic velocity measurements under helium gas pressure. Different phase transitions were identified through several elastic anomalies characterized from isobaric and isothermal sweeps. Our data reveal two crossover lines that end on the critical point terminating the first-order Mott transition line. When the critical point is approached along these lines, we observe a dramatic anomaly of the sound velocity which is consistent with a diverging compressibility of the electronic degrees of freedom.

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  • Received 6 September 2002

DOI:https://doi.org/10.1103/PhysRevLett.90.127002

©2003 American Physical Society

Authors & Affiliations

D. Fournier, M. Poirier, M. Castonguay, and K. D. Truong

  • Centre de Recherche sur les Propriétés Électroniques de Matériaux Avancés and Département de Physique, Université de Sherbrooke, Sherbrooke, Québec, Canada J1K 2R1

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Vol. 90, Iss. 12 — 28 March 2003

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