Secondary Bubble Entrainment via Primary Bubble Bursting at a Viscoelastic Surface

Bingqiang Ji, Zhengyu Yang, Zirui Wang, Randy H. Ewoldt, and Jie Feng
Phys. Rev. Lett. 131, 104002 – Published 7 September 2023
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Abstract

Bubble bursting at liquid surfaces is ubiquitous and plays a key role for the mass transfer across interfaces, impacting global climate and human health. Here, we document an unexpected phenomenon that when a bubble bursts at a viscoelastic surface of a bovine serum albumin solution, a secondary (daughter) bubble is entrapped with no subsequent jet drop ejection, contrary to the counterpart experimentally observed at a Newtonian surface. We show that the strong surface dilatational elastic stress from the viscoelastic surface retards the cavity collapse and efficiently damps out the precursor waves, thus facilitating the dominant wave focusing above the cavity nadir. The onset of daughter bubble entrainment is well predicted by an interfacial elastocapillary number comparing the effects of surface dilatational elasticity and surface tension. Our Letter highlights the important role of surface rheology on free surface flows and may find important implications in bubble dynamics with a contaminated interface exhibiting complex surface rheology.

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  • Received 25 November 2022
  • Revised 12 June 2023
  • Accepted 24 July 2023

DOI:https://doi.org/10.1103/PhysRevLett.131.104002

© 2023 American Physical Society

Physics Subject Headings (PhySH)

Fluid DynamicsPolymers & Soft Matter

Authors & Affiliations

Bingqiang Ji1,*,‡, Zhengyu Yang1, Zirui Wang1, Randy H. Ewoldt1,2,3, and Jie Feng1,3,†

  • 1Mechanical Science and Engineering, University of Illinois at Urbana-Champaign, Urbana, Illinois 61801, USA
  • 2Beckman Institute for Advanced Science and Technology, University of Illinois at Urbana-Champaign, Urbana, Illinois 61801, USA
  • 3Materials Research Laboratory, University of Illinois at Urbana-Champaign, Urbana, Illinois 61801, USA

  • *bingqiji@cityu.edu.hk
  • jiefeng@illinois.edu
  • Present address: Department of Mechanical Engineering, City University of Hong Kong, Hong Kong 999077, China.

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Issue

Vol. 131, Iss. 10 — 8 September 2023

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