Stronger Interlayer Interactions Contribute to Faster Hot Carrier Cooling of Bilayer Graphene under Pressure

Kun Ni, Jinxiang Du, Jin Yang, Shujuan Xu, Xin Cong, Na Shu, Kai Zhang, Aolei Wang, Fei Wang, Liangbing Ge, Jin Zhao, Yan Qu, Kostya S. Novoselov, Pingheng Tan, Fuhai Su, and Yanwu Zhu
Phys. Rev. Lett. 126, 027402 – Published 13 January 2021; Erratum Phys. Rev. Lett. 128, 219902 (2022)
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Abstract

We perform femtosecond pump-probe spectroscopy to in situ investigate the ultrafast photocarrier dynamics in bilayer graphene and observe an acceleration of energy relaxation under pressure. In combination with in situ Raman spectroscopy and ab initio molecular dynamics simulations, we reveal that interlayer shear and breathing modes have significant contributions to the faster hot-carrier relaxations by coupling with the in-plane vibration modes under pressure. Our work suggests that further understanding the effect of interlayer interaction on the behaviors of electrons and phonons would be critical to tailor the photocarrier dynamic properties of bilayer graphene.

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  • Received 6 July 2020
  • Revised 4 November 2020
  • Accepted 11 December 2020

DOI:https://doi.org/10.1103/PhysRevLett.126.027402

© 2021 American Physical Society

Physics Subject Headings (PhySH)

Condensed Matter, Materials & Applied Physics

Erratum

Erratum: Stronger Interlayer Interactions Contribute to Faster Hot Carrier Cooling of Bilayer Graphene under Pressure [Phys. Rev. Lett. 126, 027402 (2021)]

Kun Ni, Jinxiang Du, Jin Yang, Shujuan Xu, Xin Cong, Na Shu, Kai Zhang, Aolei Wang, Fei Wang, Liangbing Ge, Jin Zhao, Yan Qu, Kostya S. Novoselov, Pingheng Tan, Fuhai Su, and Yanwu Zhu
Phys. Rev. Lett. 128, 219902 (2022)

Authors & Affiliations

Kun Ni1,*, Jinxiang Du1,*, Jin Yang2,*, Shujuan Xu2, Xin Cong3, Na Shu1, Kai Zhang2, Aolei Wang4, Fei Wang1, Liangbing Ge1, Jin Zhao4,5, Yan Qu6, Kostya S. Novoselov7, Pingheng Tan3, Fuhai Su2,†, and Yanwu Zhu1,‡

  • 1Hefei National Research Center for Physical Sciences at the Microscale, and CAS Key Laboratory of Materials for Energy Conversion, and Department of Materials Science and Engineering, and iChEM, University of Science and Technology of China, Hefei, Anhui 230026, People’s Republic of China
  • 2Key Laboratory of Materials Physics, Institute of Solid State Physics, HFIPS, Chinese Academy of Sciences, Hefei 230031, China
  • 3State Key Laboratory of Superlattices and Microstructures, Institute of Semiconductors, Chinese Academy of Sciences, Beijing 100083, People’s Republic of China
  • 4Department of Physics, CAS Key Laboratory of Strongly-Coupled Quantum Matter Physics, and ICQD/Hefei National Laboratory for Physical Sciences at Microscale, University of Science and Technology of China, Hefei, Anhui 230026, China
  • 5Department of Physics and Astronomy, University of Pittsburgh, Pittsburgh, Pennsylvania 15260, USA and Synergetic Innovation Center of Quantum Information and Quantum Physics, University of Science and Technology of China, Hefei, Anhui 230026, China
  • 6The Sixth Element (Changzhou) Materials Technology Co., Ltd., Changzhou 213100, China
  • 7National Graphene Institute, University of Manchester, Oxford Road, Manchester M13 9PL, United Kingdom, Centre for Advanced 2D Materials, National University of Singapore, 117546 Singapore and Chongqing 2D Materials Institute, Liangjiang New Area, Chongqing 400714, China

  • *These authors contributed equally to this work.
  • To whom all correspondence should be addressed. fhsu@issp.ac.cn
  • To whom all correspondence should be addressed. zhuyanwu@ustc.edu.cn

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Vol. 126, Iss. 2 — 15 January 2021

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