Active Nonlinear Microrheology in a Glass-Forming Yukawa Fluid

D. Winter, J. Horbach, P. Virnau, and K. Binder
Phys. Rev. Lett. 108, 028303 – Published 11 January 2012

Abstract

A molecular dynamics computer simulation of a glass-forming Yukawa mixture is used to study the anisotropic dynamics of a single particle pulled by a constant force. Beyond linear response, a scaling regime is found where a force-temperature superposition principle of a Peclet number holds. In the latter regime, the diffusion dynamics perpendicular to the force can be mapped on the equilibrium dynamics in terms of an effective temperature, whereas parallel to the force a superdiffusive behavior is seen in the long-time limit. This behavior is associated with a hopping motion from cage to cage and can be qualitatively understood by a simple trap model.

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  • Received 19 September 2011

DOI:https://doi.org/10.1103/PhysRevLett.108.028303

© 2012 American Physical Society

Authors & Affiliations

D. Winter1, J. Horbach2, P. Virnau1, and K. Binder1

  • 1Institut für Physik, Johannes Gutenberg-Universität Mainz, Staudingerweg 7, 55128 Mainz, Germany
  • 2Institut für Theoretische Physik der Weichen Materie, Heinrich Heine-Universität Düsseldorf, Universitätsstraße 1, 40225 Düsseldorf, Germany

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Issue

Vol. 108, Iss. 2 — 13 January 2012

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