Magnetic Exchange Interaction between Rare-Earth and Mn Ions in Multiferroic Hexagonal Manganites

D. Talbayev, A. D. LaForge, S. A. Trugman, N. Hur, A. J. Taylor, R. D. Averitt, and D. N. Basov
Phys. Rev. Lett. 101, 247601 – Published 9 December 2008

Abstract

We report a study of magnetic dynamics in multiferroic hexagonal manganite HoMnO3 by far-infrared spectroscopy. The low-temperature magnetic excitation spectrum of HoMnO3 consists of magnetic-dipole transitions of Ho ions within the crystal-field split J=8 manifold and of the triangular antiferromagnetic resonance of Mn ions. We determine the effective spin Hamiltonian for the Ho ion ground state. The magnetic-field splitting of the Mn antiferromagnetic resonance allows us to measure the magnetic exchange coupling between the rare-earth and Mn ions.

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  • Received 4 August 2008

DOI:https://doi.org/10.1103/PhysRevLett.101.247601

©2008 American Physical Society

Authors & Affiliations

D. Talbayev1,*, A. D. LaForge2, S. A. Trugman1, N. Hur3, A. J. Taylor1, R. D. Averitt1,4, and D. N. Basov2

  • 1Center for Integrated Nanotechnologies, MS K771, Los Alamos National Laboratory, Los Alamos, New Mexico 87545, USA
  • 2Department of Physics, University of California San Diego, 9500 Gilman Drive, La Jolla, California 92093, USA
  • 3Department of Physics, Inha University, Incheon 402-751, Korea
  • 4Department of Physics, Boston University, 590 Commonwealth Avenue, Boston, Massachusetts 02215, USA

  • *diyar@lanl.gov

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Vol. 101, Iss. 24 — 12 December 2008

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