Field-induced phase diagram of the XY pyrochlore antiferromagnet Er2Ti2O7

E. Lhotel, J. Robert, E. Ressouche, F. Damay, I. Mirebeau, J. Ollivier, H. Mutka, P. Dalmas de Réotier, A. Yaouanc, C. Marin, C. Decorse, and S. Petit
Phys. Rev. B 95, 134426 – Published 18 April 2017

Abstract

We explore the field-temperature phase diagram of the XY pyrochlore antiferromagnet Er2Ti2O7 by means of magnetization and neutron diffraction experiments. Depending on the field strength and direction relative to the high symmetry cubic directions [001],[11¯0], and [111], the refined field-induced magnetic structures are derived from the zero field ψ2 and ψ3 states of the Γ5 irreducible representation which describes the ground state of XY pyrochlore antiferromagnets. At low field, domain selection effects are systematically at play. In addition, for [001], a phase transition is reported towards a ψ3 structure at a characteristic field Hc001=43 mT. For [11¯0] and [111], the spins are continuously tilted by the field from the ψ2 state, and no phase transition is found while domain selection gives rise to sharp anomalies in the field dependence of the Bragg peaks intensity. For [11¯0], these results are confirmed by high resolution inelastic neutron scattering experiments, which in addition allow us to determine the field dependence of the spin gap. This study agrees qualitatively with the scenario proposed theoretically by Maryasin et al. [Phys. Rev. B 93, 100406(R) (2016)], yet the strength of the field-induced anisotropies is significantly different from theory.

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  • Received 24 January 2017
  • Revised 24 March 2017

DOI:https://doi.org/10.1103/PhysRevB.95.134426

©2017 American Physical Society

Physics Subject Headings (PhySH)

Condensed Matter, Materials & Applied Physics

Authors & Affiliations

E. Lhotel1,*, J. Robert1, E. Ressouche2, F. Damay3, I. Mirebeau3, J. Ollivier4, H. Mutka4, P. Dalmas de Réotier2, A. Yaouanc2, C. Marin2, C. Decorse5, and S. Petit3,†

  • 1Institut Néel, CNRS and Université Grenoble Alpes, 38042 Grenoble, France
  • 2INAC, CEA and Université Grenoble Alpes, CEA Grenoble, 38054 Grenoble, France
  • 3Laboratoire Léon Brillouin, CEA, CNRS, Université Paris-Saclay, CE-Saclay, 91191 Gif-sur-Yvette, France
  • 4Institut Laue Langevin, CS 20156, 38042 Grenoble, France
  • 5ICMMO, Université Paris-Saclay, Université Paris-Sud, 91405 Orsay, France

  • *elsa.lhotel@neel.cnrs.fr
  • sylvain.petit@cea.fr

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Issue

Vol. 95, Iss. 13 — 1 April 2017

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