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Probing ultrafast spin dynamics with high-harmonic magnetic circular dichroism spectroscopy

F. Willems, C. T. L. Smeenk, N. Zhavoronkov, O. Kornilov, I. Radu, M. Schmidbauer, M. Hanke, C. von Korff Schmising, M. J. J. Vrakking, and S. Eisebitt
Phys. Rev. B 92, 220405(R) – Published 7 December 2015

Abstract

Magnetic circular dichroism in the extreme ultraviolet (XUV) spectral range is a powerful technique for element-specific probing of magnetization in multicomponent magnetic alloys and multilayers. We combine a high-harmonic generation source with a λ/4 phase shifter to obtain circularly polarized XUV femtosecond pulses for ultrafast magnetization studies. We report on simultaneously measured resonant magnetic circular dichroism (MCD) of Co and Ni at their respective M2,3 edges and of Pt at its O edge, originating from interface magnetism. We present a time-resolved MCD absorption measurement of a thin magnetic Pt/Co/Pt film, showing simultaneous demagnetization of Co and Pt on a femtosecond time scale.

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  • Received 16 September 2015
  • Revised 9 November 2015

DOI:https://doi.org/10.1103/PhysRevB.92.220405

©2015 American Physical Society

Authors & Affiliations

F. Willems1,2,*, C. T. L. Smeenk2, N. Zhavoronkov2, O. Kornilov2, I. Radu1, M. Schmidbauer3, M. Hanke4, C. von Korff Schmising1,2,†, M. J. J. Vrakking2, and S. Eisebitt1,2,*

  • 1Technische Universität Berlin, Institut für Optik und Atomare Physik, 10623 Berlin, Germany
  • 2Max-Born-Institut, Max-Born-Strasse 2A, 12489 Berlin, Germany
  • 3Leibniz-Institut für Kristallzüchtung, Max-Born-Strasse 2, 12489 Berlin, Germany
  • 4Paul-Drude-Institut für Festkörperelektronik, Hausvogteiplatz 5-7, 10117 Berlin, Germany

  • *Present address: Max-Born-Institut, Max-Born-Strasse 2A, 12489 Berlin, Germany.
  • Korff@mbi-berlin.de

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Issue

Vol. 92, Iss. 22 — 1 December 2015

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