Quantum theory of the emission spectrum from quantum dots coupled to structured photonic reservoirs and acoustic phonons

Kaushik Roy-Choudhury and Stephen Hughes
Phys. Rev. B 92, 205406 – Published 4 November 2015

Abstract

Electron-phonon coupling in semiconductor quantum dots plays a significant role in determining the optical properties of excited excitons, especially the spectral nature of emitted photons. This paper presents a comprehensive theory and analysis of emission spectra from artificial atoms or quantum dots coupled to structured photon reservoirs and acoustic phonons, when excited with incoherent pump fields. As specific examples of structured reservoirs, we chose a Lorentzian cavity and a slow-light coupled-cavity waveguide, which have both been explored experimentally. For the case of optical cavities, we directly compare and contrast the spectra from three well-known and distinct theoretical approaches to treat electron-phonon coupling, including a Markovian polaron master equation, a non-Markovian phonon correlation expansion technique, and a semiclassical linear susceptibility approach, and we point out the limitations of these models. For the cavity-QED polaron master equation, which treats the cavity-mode operator at the level of a system operator, we give closed form analytical solutions to the phonon-assisted scattering rates in the weak excitation approximation, fully accounting for temperature, cavity-exciton detuning, and cavity-dot coupling. We also show explicitly why the semiclassical linear susceptibility approach fails to correctly account for phonon-mediated cavity feeding. For weakly coupled cavities, we calculate the optical spectra using a more general photon reservoir polaron master-equation approach, and explain its differences from the above approaches in the low-Q limit of a Lorentzian cavity. We subsequently use this general reservoir approach to calculate the emission spectra from quantum dots coupled to slow-light photonic crystal waveguides, which demonstrate a number of striking photon-phonon coupling effects.

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  • Received 13 April 2015
  • Revised 1 October 2015

DOI:https://doi.org/10.1103/PhysRevB.92.205406

©2015 American Physical Society

Authors & Affiliations

Kaushik Roy-Choudhury and Stephen Hughes

  • Department of Physics, Engineering Physics & Astronomy, Queen's University, Kingston, Ontario, Canada, K7L 3N6

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Issue

Vol. 92, Iss. 20 — 15 November 2015

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