Magnons and crystal-field transitions in hexagonal RMnO3 (R = Er, Tm, Yb, Lu) single crystals

E. C. Standard, T. Stanislavchuk, A. A. Sirenko, N. Lee, and S.-W. Cheong
Phys. Rev. B 85, 144422 – Published 23 April 2012

Abstract

Far-infrared optical transmission spectra of the antiferromagnetic resonances, or magnons, and crystal-field (CF) transitions have been studied in hexagonal RMnO3 (R = Er, Tm, Yb, Lu) single crystals. The magnon and CF frequencies, their oscillator strengths, and effective g factors have been measured using external magnetic fields up to 9 T in the temperature range between 1.5 and 100 K. The magnon frequency increases systematically with a decrease of the R ion radius. The magnetic ordering of R ions (R = Er, Tm, Yb) was observed at low temperatures T<3.5 K and in strong external magnetic fields. The observed effects are analyzed taking into account the main magnetic interactions in the system including exchange of the Mn3+ spins with R3+ paramagnetic moments.

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  • Received 26 February 2012

DOI:https://doi.org/10.1103/PhysRevB.85.144422

©2012 American Physical Society

Authors & Affiliations

E. C. Standard, T. Stanislavchuk, and A. A. Sirenko*

  • Department of Physics, New Jersey Institute of Technology, Newark, New Jersey 07102, USA

N. Lee and S.-W. Cheong

  • Rutgers Center for Emergent Materials and Department of Physics and Astronomy, Rutgers University, Piscataway, New Jersey 08854, USA

  • *sirenko@njit.edu

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Issue

Vol. 85, Iss. 14 — 1 April 2012

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