Urushiol derivatives as biomass-based photocatalysts for the transition-metal-free synthesis of 1,2-amino alcohols

Xiaozhou Huang; Ya-Qing Hu; Cen Zhou; Ying Zheng; Xiao Zhang

doi:10.1039/D2GC01410F

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Urushiol derivatives as biomass-based photocatalysts for the transition-metal-free synthesis of 1,2-amino alcohols†

Xiaozhou Huang,^a Ya-Qing Hu,^a Cen Zhou,*^b Ying Zheng

^a and Xiao Zhang

*^a

Author affiliations

* Corresponding authors

^a Fujian Key Laboratory of Polymer Materials, Fujian Provincial Key Laboratory of Advanced Materials Oriented Chemical Engineering, College of Chemistry and Materials Science, Fujian Normal University, 8 Shangsan Lu, Fuzhou 350007, China
E-mail: zhangxiao@fjnu.edu.cn

^b Fujian Engineering and Research Center of New Chinese Lacquer Materials, College of Materials and Chemical Engineering, Minjiang University, Fuzhou 350108, China
E-mail: zhoucen@mju.edu.cn

Abstract

The development of catalysts from renewable and sustainable resources is an important goal in organic synthesis. Here we demonstrate the use of urushiol derivatives as biomass-based catalysts for visible-light-induced decarboxylative coupling of amino acids with aldehydes. A series of 1,2-amino alcohols are accessed in a transition-metal-free fashion under eco-friendly and redox-neutral conditions. The application of an urushiol-derived film in visible-light photoredox catalysis is also disclosed.

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Article information

DOI: https://doi.org/10.1039/D2GC01410F
Article type: Communication
Submitted: 13 Apr 2022
Accepted: 01 Jul 2022
First published: 05 Jul 2022

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Green Chem., 2022,24, 5764-5769

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Urushiol derivatives as biomass-based photocatalysts for the transition-metal-free synthesis of 1,2-amino alcohols

X. Huang, Y. Hu, C. Zhou, Y. Zheng and X. Zhang, Green Chem., 2022, 24, 5764 DOI: 10.1039/D2GC01410F

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Green Chemistry

Urushiol derivatives as biomass-based photocatalysts for the transition-metal-free synthesis of 1,2-amino alcohols†

Abstract

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Urushiol derivatives as biomass-based photocatalysts for the transition-metal-free synthesis of 1,2-amino alcohols

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