Manipulation of electronic structure via supporting ligands: a charge disproportionate model within the linear metal framework of asymmetric nickel string [Ni7(phdptrany)4Cl](PF6)

Shao-An Hua; Gin-Chen Huang; Isiah Po-Chun Liu; Jau-Huei Kuo; Ching-Hong Jiang; Chien-Lan Chiu; Chen-Yu Yeh; Gene-Hsiang Lee; Shie-Ming Peng

doi:10.1039/B926315B

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Manipulation of electronic structure via supporting ligands: a charge disproportionate model within the linear metal framework of asymmetric nickel string [Ni₇(phdptrany)₄Cl](PF₆)†

Shao-An Hua,^a Gin-Chen Huang,^a Isiah Po-Chun Liu,‡^ab Jau-Huei Kuo,^a Ching-Hong Jiang,^a Chien-Lan Chiu,^c Chen-Yu Yeh,^c Gene-Hsiang Lee^a and Shie-Ming Peng*^ab

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* Corresponding authors

^a Department of Chemistry, National Taiwan University, Taipei, Taiwan, ROC
E-mail: smpeng@ntu.edu.tw
Fax: (+886)2-8369-3765

^b Institute of Chemistry, Academia Sinica, Taipei, 115, Taiwan, ROC

^c Department of Chemistry, National Chung Hsing University, Taichung, Taiwan

Abstract

This paper describes the synthesis and physical properties of an uniquely asymmetric heptanickel string complex exhibiting a charge disproportionate model along the linear nickel framework.

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Article information

DOI: https://doi.org/10.1039/B926315B
Article type: Communication
Submitted: 14 Dec 2009
Accepted: 13 May 2010
First published: 04 Jun 2010

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Chem. Commun., 2010,46, 5018-5020

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Manipulation of electronic structure via supporting ligands: a charge disproportionate model within the linear metal framework of asymmetric nickel string [Ni₇(phdptrany)₄Cl](PF₆)

S. Hua, G. Huang, I. P. Liu, J. Kuo, C. Jiang, C. Chiu, C. Yeh, G. Lee and S. Peng, Chem. Commun., 2010, 46, 5018 DOI: 10.1039/B926315B

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Chemical Communications