A non-chemically selective top-down approach towards the preparation of hierarchical TS-1 zeolites with improved oxidative desulfurization catalytic performance

Shuting Du; Xiaoxin Chen; Qiming Sun; Ning Wang; Mingjun Jia; Valentin Valtchev; Jihong Yu

doi:10.1039/C5CC10232D

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A non-chemically selective top-down approach towards the preparation of hierarchical TS-1 zeolites with improved oxidative desulfurization catalytic performance†

Shuting Du,‡^a Xiaoxin Chen,‡^a Qiming Sun,^a Ning Wang,^a Mingjun Jia,^b Valentin Valtchev^ac and Jihong Yu*^a

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* Corresponding authors

^a State Key Laboratory of Inorganic Synthesis and Preparative Chemistry, College of Chemistry, Jilin University, Changchun 130012, P. R. China
E-mail: jihong@jlu.edu.cn

^b Key Laboratory of Surface and Interface Chemistry of Jilin Province, College of Chemistry, Jilin University, Changchun 130012, P. R. China

^c Laboratory of Catalysis and Spectrochemistry, University of Normandy, 6 boulevard Marechal Juin, 14050 Caen, France

Abstract

Hierarchical TS-1 zeolites with secondary macropores have been successfully prepared by using two different fluoride-containing chemical etching post-treated routes. Hierarchical TS-1 zeolites exhibited a chemical composition similar to that of the parent material and showed remarkably enhanced catalytic activity in oxidative desulfurization reaction.

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Article information

DOI: https://doi.org/10.1039/C5CC10232D
Article type: Communication
Submitted: 12 Dec 2015
Accepted: 28 Jan 2016
First published: 28 Jan 2016

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Chem. Commun., 2016,52, 3580-3583

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A non-chemically selective top-down approach towards the preparation of hierarchical TS-1 zeolites with improved oxidative desulfurization catalytic performance

S. Du, X. Chen, Q. Sun, N. Wang, M. Jia, V. Valtchev and J. Yu, Chem. Commun., 2016, 52, 3580 DOI: 10.1039/C5CC10232D

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Chemical Communications

A non-chemically selective top-down approach towards the preparation of hierarchical TS-1 zeolites with improved oxidative desulfurization catalytic performance†

Abstract

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A non-chemically selective top-down approach towards the preparation of hierarchical TS-1 zeolites with improved oxidative desulfurization catalytic performance

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