Abstract
Methane can be converted in high yields to aromatic products using an integrated recycle system containing both an oxidative coupling (OCM) reactor at 800°C, for conversion of CH4 to C2H4, and a secondary reactor containing Ga/ZSM-5 at 520°C for subsequent conversion of ethylene to aromatics. Using this system, aromatic product yields of >70% at CH4 conversions of ~100%, based on total CH4 added, can be obtained.
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Qiu, P., Lunsford, J. & Rosynek, M. Steady-state conversion of methane to aromatics in high yields using an integrated recycle reaction system. Catalysis Letters 48, 11–15 (1997). https://doi.org/10.1023/A:1019031205308
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DOI: https://doi.org/10.1023/A:1019031205308