Skip to main content
Log in

Source apportionment for urban PM10 and PM2.5 in the Beijing area

  • Articles
  • Published:
Chinese Science Bulletin

Abstract

Airborne particulate matter (PM2.5 and PM10) samples were collected at the Beijing Normal University sampling site in the urban area of Beijing, China in dry and wet seasons during 2001–2004. Concentrations of 23 elements and 14 ions in particulate samples were determined by ICP-AES and IC, respectively. Source apportionment results derived from both Positive Matrix Factorization (PMF) and Chemical Mass Balance (CMB) models indicate that the major contributors of PM2.5 and PM10 in Beijing are: soil dust, fossil fuel combustion, vehicle exhausts, secondary particulate, biomass burning and some industrial sources. We have identified both regional common sources, such as vehicular emissions, particulate of secondary origin and biomass burning, as well as country-specific problems, such as sand storms and soil dust that should be addressed for effective air quality control.

This is a preview of subscription content, log in via an institution to check access.

Access this article

Price excludes VAT (USA)
Tax calculation will be finalised during checkout.

Instant access to the full article PDF.

Similar content being viewed by others

References

  1. BEPB (Beijing Municipal Environmental Protection Bureau). Communique on the Environmental Status in Beijing in 2002 (in Chinese). Beijing Municipal Environmental Protection Bureau, 2003

  2. Chameides W L, Yu H, Liu S C, et al. Case study of the effects of atmospheric aerosols and regional haze on agriculture: an opportunity to enhance crop yields in China through emission controls. Proc Nat Acad Sci USA, 1999, 96(24): 13626–13633

    Article  Google Scholar 

  3. Winchester J W, Bi M. Fine and coarse aerosol composition in an urban setting: a case study in Beijing. Atmospheric Environment, 1984, 18(7): 1399–1409

    Article  Google Scholar 

  4. Yang S J, Yang Y N, Qian Q F, et al. Characteristics of airborne particulate and identification of their sources in Beijing-Tianjin area. Acta Sci Circumstant (in Chinese), 1987, 7(4): 411–423

    Google Scholar 

  5. Dong J Q, Yang S J. Characteristics of the aerosol and study of their sources in Huabei clean area. Environ Chem (in Chinese), 1998, 17(1): 38–44

    Google Scholar 

  6. Wang W, Tang D G, Liu H J. Research on current pollution status and characteristics of PM2.5 in China. Res Environ Sci (in Chinese), 2000, 13(1): 1–5

    Google Scholar 

  7. Chen Z, Ge S, Zhang J. Measurement and analysis for atmospheric aerosol particulates in Beijing. Res Environ Sci (in Chinese), 1994, 7(3): 1–9

    Google Scholar 

  8. Yao X, Chan C K, Fang M, Cadle S. The water-soluble ionic composition of PM2.5 in Shanghai and Beijing, China. Atmos Environ, 2002, 36(26): 4223–4234

    Article  Google Scholar 

  9. Yao X, Lau A P S, Fang M, Chan C K. Size distribution and formation of ionic species in atmospheric particulate pollutants in Beijing, China: 1-inorganic ions. Atmos Environ, 2003, 37: 2991–3000

    Article  Google Scholar 

  10. He K B, Yang F M, Ma Y L, et al. The characteristics of PM2.5 in Beijing, China. Atmos Environ, 2001, 35: 4959–4970

    Article  Google Scholar 

  11. Yao X H, Lau A P S, Fang M, et al. Size distributions and formation of ionic species in atmospheric particulate pollutants in Beijing, China: 2-dicarboxylic acids. Atmos Environ, 2003, 37: 3001–3002

    Article  Google Scholar 

  12. Dan M, Zhuang G S, Li X X, et al. The characteristics of carbonaceous species and their sources in PM2.5 in Beijing. Atmos Environ, 2004, 38: 3443–3452

    Article  Google Scholar 

  13. He L Y, Hu M, Huang X F, et al. Measurement of emissions of fine particulate organic matter from Chinese cooking. Atmos Environ, 2004, 38: 6557–6564

    Article  Google Scholar 

  14. Wang Y, Zhuang G S, Tang A H, et al. The ion chemistry and the sources of PM2.5 aerosol in Beijing. Atmos Environ, 2005, 39: 3771–3784

    Article  Google Scholar 

  15. Huang X F, Hu M, He LY, et al. Chemical characterization of water-soluble organic acids in PM2.5 in Beijing, China. Atmos Environ, 2005, 39: 2819–2927

    Article  Google Scholar 

  16. Yang F M, Ye B M, He K B, et al. Characterisation of atmospheric mineral compounds of PM2.5 in Beijing and Shanghai. Sci Total Environ, 2005, 343: 221–230

    Article  Google Scholar 

  17. Duan F K, He K B, Ma Y L, et al. Concentration and chemical characteristics of PM2.5 in Beijing, China. Sci Total Environ, 2006, 355: 264–275

    Article  Google Scholar 

  18. Feng J L, Hu M, Chan C K, et al. A comparative study of the organic matter in PM2.5 from three China megacities in three different climatic zones. Atmos Environ, 2006, 40: 3983–3994

    Article  Google Scholar 

  19. Huang X F, He L Y, Hu M, et al. Annual variation of particulate organic compounds in PM2.5 in the urban atmosphere of Beijing. Atmos Environ, 2006, 40: 2449–2458

    Article  Google Scholar 

  20. Sun Y L, Zhuang G S, Wang Y, et al. The air-borne particulate pollution in Beijing— concentration, composition, distribution and sources. Atmos Environ, 2004, 38: 5991–6004

    Article  Google Scholar 

  21. Yuan H, Wang Y, Zhuang G. The simultaneous determination of organic acid, MSA with inorganic anions in aerosol and rain-water by ion chromatography. J Instrum Anal (in Chinese), 2003, 6: 12–16

    Google Scholar 

  22. Paatero P. User’s Guide for Positive Matrix Factorization Programs PMF2 and PMF3. Helsinki: University of Helsinki, 1998

    Google Scholar 

  23. Ramadan Z, Song X H, Hopke P K. Identification of source of Phoenix aerosol by positive matrix factorization. J Air & Waste Manag Assoc, 2000, 50: 1308–1320

    Google Scholar 

  24. Hiena P D, Bacb V T, Thinhb N T H, et al. PMF receptor modeling of fine and coarse PM10 in air masses governing monsoon conditions in Hanoi, Northern Vietnam. Atmos Environ, 2004, 38: 189–201

    Article  Google Scholar 

  25. Kima E, Larsonb T V, Hopke P K, et al. Source identification of PM2.5 in an arid Northwest U.S. City by positive matrix factorization. Atmos Res, 2003, 66: 291–305

    Article  Google Scholar 

  26. Watson J G, Robinson N F, Lewis C, et al. Chemical mass balance receptor model version 8, (CMB8) User’s Manual, Desert Research Institute Document No. 1808.1D1, Desert Research Institute, 1997

  27. USEPA, USEPA Speciate: VOC/PM speciation data system, User’s Manual, Version 3.1, USEPA, 1997

  28. Ge S. Beijing aerosol characterization study: Influence of coal burning. Dissertation for the degree of Ph. D. submitted to the Oregon Graduate Institute of Science & Technology, University Microfilm International, DA9238754, 1992, 185

Download references

Author information

Authors and Affiliations

Authors

Corresponding author

Correspondence to Hao ZhengPing.

Additional information

Supported by the Swedish International Development Cooperation Agency (SIDA), and coordinated by the Asian Institute of Technology

About this article

Cite this article

Zhang, W., Guo, J., Sun, Y. et al. Source apportionment for urban PM10 and PM2.5 in the Beijing area. CHINESE SCI BULL 52, 608–615 (2007). https://doi.org/10.1007/s11434-007-0076-5

Download citation

  • Received:

  • Accepted:

  • Issue Date:

  • DOI: https://doi.org/10.1007/s11434-007-0076-5

Keywords

Navigation