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Lead-free (0.93 − x)Bi0.5Na0.5TiO3–0.07BaTiO3–xNaNbO3 relaxor ferroelectrics for energy storage applications

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Abstract

In this work, (0.93 − x)Bi0.5Na0.5TiO3–0.07BaTiO3–xNaNbO3 (BNT–0.07BT–xNN) lead-free energy storage ceramics were designed on the basis of the phase diagram of this system. The phase structure and energy storage property were studied. The NN substitution into BNT–BT increased the crystal structure symmetry and induced an obvious disruption of the ferroelectric order. At x = 0.20, an extremely slim P–E hysteresis loop along with a large recoverable energy storage density (Wrec) of 2.08 J/cm3 and a high energy storage effificiency (η) of 81% was obtained at a moderate electric field of 160 kV/cm. The BNT–BT–0.02NN ceramic possessed a high discharge energy density (Wd ~ 1.44 J/cm3) and a fast discharge speed (t0.9 ~ 153 ns) at an electric field of 160 kV/cm. These results show that the BNT–0.07BT–xNN material may be a promising candidate for capacitors.

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Acknowledgements

This work was supported by the Innovation Team of Higher Educational Science and Technology Program in Shandong Province (No. 2019KJA025), National Natural Science Foundation of China (No. 51701091). Natural Science Foundation of Shandong Province of China (Nos. ZR2018MEM011 and ZR201709270099), Opening Project of Key Laboratory of Inorganic Functional Materials and Devices, Chinese Academy of Sciences (Grant No. KLIFMD201705), Research Foundation of Liaocheng University (No.318011906), State Key Laboratory of New Ceramic and Fine Processing Tsinghua University (No. KF201906), The National Undergraduate Training Programs for Innovation and Entrepreneurship of China (No. 201910447002), and The Undergraduate Training Programs for Innovation and Entrepreneurship of Liaocheng University (No. cxcy2019y002).

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Authors and Affiliations

  1. School of Materials Science and Engineering, Liaocheng University, Liaocheng, 252059, China

    Bingkai Chu, Xu Tang, Jigong Hao, Peng Li, Peng Fu, Chong Chen & Wei Li

  2. The State Key Lab of High Performance Ceramics and Superfinemicrostructure, Shanghai Institute of Ceramics, Chinese Academy of Science, Shanghai, 200050, People’s Republic of China

    Guorong Li

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  1. Bingkai Chu
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Correspondence to Jigong Hao or Wei Li.

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Chu, B., Tang, X., Hao, J. et al. Lead-free (0.93 − x)Bi0.5Na0.5TiO3–0.07BaTiO3–xNaNbO3 relaxor ferroelectrics for energy storage applications. J Mater Sci: Mater Electron 31, 22676–22686 (2020). https://doi.org/10.1007/s10854-020-04779-5

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