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Synthesis and characterization of Bi0.5Na0.5TiO3-BaTiO3-K0.5Na0.5NbO3 ceramics for energy storage applications

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Abstract

Structural, microstructural, dielectric, ferroelectric and piezoelectric properties of the (0.95-x)Bi0.5Na0.5TiO3–0.05BaTiO3-xK0.5Na0.5NbO3 (BNT-BT-KNN) lead-free ceramics with 0.0 ≤ x ≤ 0.06 were studied. Samples were synthesized through the mechanochemically activated solid-state method and structurally characterized by X-ray diffraction (XRD) and Raman-spectroscopic studies, whereas the microstructure of all samples was analyzed by Field Emission Scanning Electron Microscopy (FE-SEM). When KNN concentration and temperature were increased, the transition from a ferroelectric to relaxor state was detected by ferroelectric-loop measurements. Furthermore, the high-energy storage efficiency values at room temperature obtained for samples with x ≥ 0.04 confirm the suitability of these ceramics for energy storage applications.

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Acknowledgments

The authors thank University of Mar del Plata (Argentina) Project (15G/388) and National Agency for Scientific and Technological Promotion (ANPCyT) PICT 2014-1314 for providing financial support.

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Authors and Affiliations

  1. Institute of Research in Materials Science and Technology (INTEMA), Av. Colón 10850, B7606BWV, Mar del Plata, Argentina

    A. Prado, J. Camargo, L. Ramajo & M. Castro

  2. Department of Materials Science and Engineering, Friedrich Alexander Universität Erlangen-Nürnberg, Martensstr.5, 91058, Erlangen, Germany

    P. Öchsner

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  1. A. Prado
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  2. J. Camargo
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  3. P. Öchsner
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  4. L. Ramajo
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Correspondence to M. Castro.

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Prado, A., Camargo, J., Öchsner, P. et al. Synthesis and characterization of Bi0.5Na0.5TiO3-BaTiO3-K0.5Na0.5NbO3 ceramics for energy storage applications. J Electroceram 44, 248–255 (2020). https://doi.org/10.1007/s10832-020-00216-5

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