Skip to main content

Advertisement

Log in

Distribution and sources of polycyclic aromatic hydrocarbons in Wuhan section of the Yangtze River, China

  • Published:
Environmental Monitoring and Assessment Aims and scope Submit manuscript

Abstract

Polycyclic aromatic hydrocarbons (PAHs) are important organic contaminants with great significance for China, where coal burning is the main source of energy. In this study, concentrations, distribution between different phases, possible sources and eco-toxicological effect of PAHs of the Yangtze River were assessed. PAHs in water, suspended particulate matters (SPM) and sediment samples at seven main river sites, 23 tributary and lake sites of the Yangtze River at the Wuhan section were analyzed. The total concentrations of PAHs in the studied area ranged from 0.242 to 6.235 μg/l in waters and from 31 to 4,812 μg/kg in sediment. The average concentration of PAHs in SPM was 4,677 μg/kg, higher than that in sediment. Benzo(a)pyrene was detected only at two stations, but the concentrations were above drinking water standard. The PAHs level of the Yangtze River was similar to that of some other rivers in China but higher than some rivers in foreign countries. There existed a positive relationship between PAHs concentrations and the TOC contents in sediment. The ratio of specific PAHs indicated that PAHs mainly came from combustion process, such as coal and wood burning. PAHs may cause potential toxic effect but will not cause acute biological effects in sedimentary environment of the Wuhan section of the Yangtze River.

This is a preview of subscription content, log in via an institution to check access.

Access this article

Price excludes VAT (USA)
Tax calculation will be finalised during checkout.

Instant access to the full article PDF.

Similar content being viewed by others

References

  • Chiou, C. T., Porter, P. E., & Schmeddling, D. W. (1983). Partition equilibria of nonionic organic compounds between soil organic matter and water. Environmental Science & Technology, 17, 227–231.

    Article  CAS  Google Scholar 

  • Doong, R., & Lin, Y. T. (2004). Characterization and distribution of polycyclic aromatic hydrocarbon contaminations in surface sediment and water from Gao-ping River, Taiwan. Water Research, 38, 1733–1744.

    Article  CAS  Google Scholar 

  • Fernandes, M. B., Sicre, M. A., Boireau, A., & Tronszynski, J. (1997). Polyaromatic hydrocarbon (PAH) distributions in the Seine River and its estuary. Marine Pollution Bulletin, 34, 857–867.

    Article  CAS  Google Scholar 

  • Forster, G. D., & Wrighrt, D. A. (1988). Unsubstitute polycyclic aromatic hydrocarbons in sediments, clams, and clam worms from Chesapeake Bay. Marine Pollution Bulletin, 19, 459–465.

    Article  Google Scholar 

  • Hong, H., Xu, L., Zhang, L., Chen, J. C., Wong, Y. S., & Wan, T. S. M. (1995). Environmental fate chemistry of organic pollutions in the sediment of Xiamen and Victoria Habours. Marine Pollution Bulletin, 31, 229–236.

    Article  CAS  Google Scholar 

  • Hubei Statistical Bureau (2005). Statistical yearbook of Hubei province. Beijing: China Statistical Press.

    Google Scholar 

  • International Organization for Standardization (1998). ISO13877: Soil quality determination of polynuclear aromatic hydrocarbons-method using high-performance liquid chromatography.

  • Jiang, X., Xu, S. F., Martens, D., & Wang, L. S. (2000). Polychlorinated organic contaminants in waters, suspended solids and sediments of the Nanjing section, Yangtze River. China Environmental Science, 20(3), 193–197.

    Google Scholar 

  • Kim, G. B., Maruya, K. A., Lee, K. A., Lee, R. F., Lee, J. H., Koh, C. H., et al. (1999). Distribution and sources of polycyclic aromatic hydrocarbons in sediments from Kyeonggi Bay, Korea. Marine Pollution Bulletin, 38, 7–15.

    Article  CAS  Google Scholar 

  • Li, G. C., Xia, X. H., & Yang, Z. F. (2006). Distribution and sources of polycyclic aromatic hydrocarbons in the middle and lower reaches of the Yellow River, China. Environmental Pollution, 144, 985–993.

    Article  CAS  Google Scholar 

  • Liu, M., Hou, L. J., Zou, H. X., Yang, Y., Lu, J. H., & Wang, X. R. (2001). Distribution characteristics of polycyclic aromatic hydrocarbons (PAHs) in surface sediments of tidal flats of the Yangtze Estuary. China Environmental Science, 21(4), 343–346.

    CAS  Google Scholar 

  • Liu, H. L., Liu, M., Cheng, S. B., & Ou, D. N. (2005). Occurrence of organochlorine pesticides (OCPs) in suspended particle matters (SPMs) and surface sediments of the south bank of the Yangtze estuary. China Environmental Science, 25(5), 622–626.

    CAS  Google Scholar 

  • Long, E. R., MacDonald, D. D., Smith, S. L., & Calder, F. D. (1995). Incidence of adverse biological effects within range of chemical concentrations in marine and estuary sediment. Environmental Management, 19, 81–97.

    Article  Google Scholar 

  • Macias-Zamora, J. V., Mendoza-Vega, E., & Villaescusa-Celaya, J. A. (2002). PAHs composition of surface marine sediments: A comparison to potential local sources in Todos Santos Bay, BC, Mexico. Chemosphere, 46, 459–468.

    Article  CAS  Google Scholar 

  • Mai, B. X., Fu, J. M., Sheng, G. Y., Kang, Y. H., Lin, Z., Zhang, G., et al. (2002). Chlorinated and polycyclic aromatic hydrocarbons in riverine and estuarine sediments from Pearl River Delta, China. Environmental Pollution, 117, 457–474.

    Article  CAS  Google Scholar 

  • Mai, B. X., Fu, J. M., Zhang, G., Lin, Z., Min, Y. S., Sheng, G. Y., et al. (2001). Polycyclic aromatic hydrocarbons in sediments from the Pearl River and estuary, China: Spatial and temporal distribution and sources. Applied Geochemistry, 16(11, 12), 1429–1445.

    Google Scholar 

  • Manoli, E., & Samara, C. (1999). Polycyclic aromatic hydrocarbons in natural waters: Sources, occurrence and analysis. Trends in Analytical Chemistry, 18(6), 417–428.

    Article  CAS  Google Scholar 

  • Maskaoui, K., Zhoub, J. L., Hong, H. S., & Zhang, Z. L. (2002). Contamination by polycyclic aromatic hydrocarbons in the Jiulong River Estuary and Western Xiamen Sea, China. Environmental Pollution, 118, 109–122.

    Article  CAS  Google Scholar 

  • Mitra, S., & Bianchi, T. S. (2003). A preliminary assessment of polycyclic aromatic hydrocarbon distributions in the lower Mississippi River and Gulf of Mexico. Marine Chemistry, 82, 273–288.

    Article  CAS  Google Scholar 

  • Notar, M., Leskovsek, H., & Faganeli, J. (2001). Composition, distribution and sources of polycyclic aromatic hydrocarbons in sediments of the Gulf of Trieste, Northern Adriatic Sea. Marine Pollution Bulletin 42(1), 36–44.

    Article  CAS  Google Scholar 

  • Shi, Z., Tao, S., Pan, B., Fan, W., He, X. C., Zuo, Q., et al. (2005). Contamination of rivers in Tianjin, China by Polycyclic aromatic hydrocarbons. Environmental Pollution, 134, 97–111.

    Article  CAS  Google Scholar 

  • Simpson, C. D., Mosi, A. A., Cullen, W. R., & Reimer, K. J. (1996). Composition and distribution of polycyclic in surficial marine sediments from Kitimat Harbour, Canada. Science of the Total Environment, 181, 265–278.

    Article  CAS  Google Scholar 

  • Soclo, H. H., Garrigues, P. H., & Ewald, M. (2000). Origin of polycyclic aromatic hydrocarbons (PAHs) in coastal marine sediments: Case studies in Cotonou (Benin) and Aquitaine (France) areas. Marine Pollution Bulletin, 40(5), 387–396.

    Article  CAS  Google Scholar 

  • State Environmental Protection Administration of China (SEPA) (2002a). Monitoring and analytical method on water and waste water (4th edn.). Beijing: China Environmental Science Press.

    Google Scholar 

  • State Environmental Protection Administration of China (SEPA) (2002b). GB3838-2002: Environmental Quality Standard for Surface Water.

  • State standard of China (GB13198-91):Water quality-determination of specified six polynuclear aromatic hydrocarbons-high performance liquid chromatography.

  • Witt, G. (1995). Polycyclic aromatic hydrocarbons in water and sediment of the Baltic Sea (Alaska). Marine Pollution Bulletin, 31, 237–248.

    Article  CAS  Google Scholar 

  • Xiong, J. H., Gan, D. A., & Luo, Y. S. (2004). The function of Wuhan city in the Wuhan economic circle. Territory & Natural Resources Study, 3, 8–10.

    Google Scholar 

  • Xu, S. F., Jiang, X., Wang, L. S., Quan, X., & Martens, D. (2000). Polycyclic aromatic hydrocarbons (PAHs) pollutants in sediments of the Yangtze River and the Liao River. China Environmental Science, 20(2), 128–131.

    CAS  Google Scholar 

  • Yunker, M. B., Macdonald, R. W., Vingarzan, R., Mitchell, R. H., Goyette, D., & Sylvestre, S. (2002). PAHs in the Fraser River basin: A critical appraisal of PAH ratios as indicators of PAH source and composition. Organic Geochemistry, 33, 489–515.

    Article  CAS  Google Scholar 

  • Zakaria, M. P., Takada, H., Tsutsumi, S., Ohno, K., Yamada, J., Kouno, E., et al. (2002). Distribution of polycyclic aromatic hydrocarbons (PAHs) in rivers and estuaries in Malaysia: A widespread input of petrogenic PAHs. Environmental Science & Technology, 36, 1907–1918.

    Article  CAS  Google Scholar 

  • Zhang, Z. L., Huang, J., Yu, G., & Hong, H. S. (2004). Occurrence of PAHs, PCBs and organochlorine pesticides in the Tonghui River of Beijing, China. Environmental Pollution, 130, 249–261.

    Article  CAS  Google Scholar 

  • Zhou, J. L., & Maskaoui, K. (2003). Distribution of polycyclic aromatic hydrocarbons in water and surface sediments from Daya Bay, China. Environmental Pollution, 121, 269–281.

    Article  CAS  Google Scholar 

  • Zhu, L. Z., Chen, B. L., & Wang, J. (2004). Pollution survey of polycyclic aromatic hydrocarbons in surface water of Hangzhou, China. Chemosphere, 56, 1085–1095.

    Article  CAS  Google Scholar 

Download references

Author information

Authors and Affiliations

Authors

Corresponding author

Correspondence to Xinghui Xia.

Rights and permissions

Reprints and permissions

About this article

Cite this article

Feng, C., Xia, X., Shen, Z. et al. Distribution and sources of polycyclic aromatic hydrocarbons in Wuhan section of the Yangtze River, China. Environ Monit Assess 133, 447–458 (2007). https://doi.org/10.1007/s10661-006-9599-5

Download citation

  • Received:

  • Accepted:

  • Published:

  • Issue Date:

  • DOI: https://doi.org/10.1007/s10661-006-9599-5

Keywords

Navigation