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Neutron Scattering in Layered Copper-Oxide Superconductors pp 225–260Cite as

Phase Separation, Charge Segregation, and Superconductivity in Layered Cuprates

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Part of the book series: Physics and Chemistry of Materials with Low-Dimensional Structures ((PCMALS,volume 20))

Abstract

Experimental observations suggesting inhomogeneity in the layered cuprates have been reported since shortly after the discovery of superconductivity in these materials [1]. There are at least two forms of inhomogeneity that have, by now, been fairly well established. One involves the phase separation of oxygen interstitials in La2CuO4+δ . The interstitials are mobile near room temperature, giving a homogeneous phase, while cooling to lower temperatures can lead to segregation into phases with distinct oxygen concentrations. Early work focussed on samples with δ < 0.05, in which case the two phases present at low temperature are the nearly-stoichiometric an-tiferromagnet (described in Chapter 4) and an oxygen-rich superconducting phase. For larger δ, multiple superconducting phases have been discovered, with the T c varying with δ. It has also been shown that, within a particular oxygen-rich phase, the interstitials order in a layered fashion. Neutron diffraction has played a crucial role in establishing the nature of phase separation and order in La2CuO4+δ , and that work is the subject of the first half of this chapter.

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  1. Brookhaven National Laboratory, Upton, NY, 11913, USA

    J. M. Tranquada

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  1. Laboratory for Neutron Scattering, ETH Zurich & Paul Scherrer Institute, Villigen PSI, Switzerland

    Albert Furrer

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Tranquada, J.M. (1998). Phase Separation, Charge Segregation, and Superconductivity in Layered Cuprates. In: Furrer, A. (eds) Neutron Scattering in Layered Copper-Oxide Superconductors. Physics and Chemistry of Materials with Low-Dimensional Structures, vol 20. Springer, Dordrecht. https://doi.org/10.1007/978-94-015-1284-8_6

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  • DOI: https://doi.org/10.1007/978-94-015-1284-8_6

  • Publisher Name: Springer, Dordrecht

  • Print ISBN: 978-90-481-5091-5

  • Online ISBN: 978-94-015-1284-8

  • eBook Packages: Springer Book Archive

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