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Organic/Inorganic Composite Latexes: The Marriage of Emulsion Polymerization and Inorganic Chemistry

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Hybrid Latex Particles

Part of the book series: Advances in Polymer Science ((POLYMER,volume 233))

Abstract

This review article describes recent advances in the synthesis and properties of waterborne organic/inorganic colloids elaborated through conventional emulsion polymerization, a well-established technology. These materials can be defined as aqueous suspensions of composite latex particles made up of organic and inorganic domains organized into well-defined core–shell, multinuclear, raspberry-like, multipod-like, or armored morphologies. Particular emphasis is placed on the synthetic strategies for fabrication of these colloidal materials. Two main approaches are described: the polymerization of organic monomers in the presence of preformed inorganic particles, and the reverse approach by which inorganic materials are synthesized in the presence of preformed polymer latexes. The list of examples provided in this review is by no means exhaustive but rather intends to give an overview of synthetic methods for selected inorganic compounds (e.g., silica, iron oxide, pigments, clays, quantum dots, and metals), and briefly reports on potential applications of the resulting materials.

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Abbreviations

1VID:

1-Vinylimidazole

2VPy:

2-Vinylpyridine

4VPy:

4-Vinylpyridine

AA:

Acrylic acid

AAEM:

Acetoacetoxyethyl methacrylate

AAm:

Acrylamide

ACPA:

4,4′-Azobis(4-cyanopentanoic acid)

AEMH:

2-Aminoethylmethacrylamide hydrochloride

AFM:

Atomic force microscopy

AIBA:

2,2′-Azobis(2-amidinopropane) dihydrochloride

AIBN:

2,2′-Azobis(isobutyronitrile)

AOA:

12-Acryloxy-9-octadecenoic acid

BA:

n-Butyl acrylate

BMA:

n-Butyl methacrylate

CMC:

Critical micelle concentration

CS:

Chitosan

CTAB:

Cetyltrimethyl ammonium bromide

DMAEMA:

N,N-Dimethylaminoethyl methacrylate

DSC:

Differential scanning calorimetry

DVB:

Divinyl benzene

EGDMA:

Ethylene glycol dimethacrylate

GA:

Gluteraldehyde

GMA:

Glycidyl methacrylate

HEMA:

2-Hydroxyethyl methacrylate

KPS:

Potassium persulfate

MA:

Maleic anhydride

MAA:

Methacrylic acid

MADQUAT:

2-Methacryloyloxy ethyl trimethyl ammonium chloride

MBA:

N,N ′-Methylene bisacrylamide

MMA:

Methyl methacrylate

MMT:

Montmorillonite

MPDES:

Methacryloxy propyl dimethyl ethoxysilane

MPDMS:

Methacryloxy propyl dimethoxysilane

MPTMS:

Methacryloxy propyl trimethoxysilane

MTC:

2-(Methacryloyl) ethyl trimethyl ammonium chloride

Ms:

Saturation magnetization

NaSS:

Sodium styrene sulfonate

NIPAM:

N-Isopropylacrylamide

NVCL:

N-Vinylcaprolactam

OA:

Oleic acid

O/I:

Organic/inorganic

P4VPy:

Poly(4-vinylpiridine)

P2VPy:

Poly(2-vinylpiridine)

PCN:

Polymer–clay nanocomposites

PEG:

Poly(ethylene glycol)

PEGMA:

Poly(ethylene glycol) monomethyl ether methacrylate

PMMA:

Poly(methyl methacrylate)

PS:

Polystyrene

PSD:

Particle size distribution

PVA:

Polyvinyl alcohol

PVP:

Poly(N-vinylpyrrolidone)

QDs:

Quantum dots

S:

Styrene

SDBS:

Sodium dodecylbenzene sulfonate

SDS:

Sodium dodecyl sulfate

SEM:

Scanning electron microscopy

TEM:

Transmission electron microscopy

TEOS:

Tetraethyl orthosilicate

T g :

Glass transition temperature

TGA:

Thermogravimetric analysis

VDAC:

Vinylbenzyl dimethyl dodecyl ammonium chloride

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  1. Univ. Lyon 1, CPE Lyon, CNRS UMR5265, Laboratoire de Chimie, Catalyse, Polymères et Procédés (C2P2), LCPP team, Université de Lyon, 43 Bd du 11 Novembre 1918, 69616, Villeurbanne, France

    Elodie Bourgeat-Lami & Muriel Lansalot

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  1. Dept. Chemical Engineering & Chemistry, Eindhoven University of Technology, Eindhoven, Netherlands

    Alex M. van Herk

  2. Max-Planck-Institute for Polymer Researc, Ackermannweg 10, Mainz, 55128, Germany

    Katharina Landfester

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Bourgeat-Lami, E., Lansalot, M. (2010). Organic/Inorganic Composite Latexes: The Marriage of Emulsion Polymerization and Inorganic Chemistry. In: van Herk, A., Landfester, K. (eds) Hybrid Latex Particles. Advances in Polymer Science, vol 233. Springer, Berlin, Heidelberg. https://doi.org/10.1007/12_2010_60

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