Exploring quantum control landscape structure

Arun Nanduri, Ashley Donovan, Tak-San Ho, and Herschel Rabitz
Phys. Rev. A 88, 033425 – Published 30 September 2013

Abstract

A common goal of quantum control is to maximize a physical observable through the application of a tailored field. The observable value as a function of the field constitutes a quantum-control landscape. Previous papers have shown, under specified conditions, that the quantum-control landscape should be free of suboptimal critical points. This favorable landscape topology is one factor contributing to the efficiency of climbing the landscape. An additional complementary factor is the landscape structure, which constitutes all nontopological features. If the landscape's structure is too complex, then climbs may be forced to take inefficient convoluted routes to find optimal controls. This paper provides a foundation for understanding control-landscape structure by examining the linearity of gradient-based optimization trajectories through the space of control fields. For this assessment, a metric R1 is defined as the ratio of the path length of the optimization trajectory to the Euclidean distance between the initial control field and the resultant optimal control field that takes an observable from the bottom to the top of the landscape. Computational analyses for simple model quantum systems are performed to ascertain the relative abundance of nearly straight control trajectories encountered when optimizing a state-to-state transition probability. The distribution of R values is found to be centered near remarkably low values upon sampling large numbers of randomly chosen initial control fields. Additionally, a stochastic algorithm is used to locate many distinct initial control fields, each of which corresponds to the start of an almost straight control trajectory with R1.0. The collected results indicate that quantum-control landscapes have very simple structural features. The favorable topology and the complementary simple structure of the control landscape provide a basis for understanding the generally observed ease of optimizing a state-to-state transition probability.

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  • Received 19 May 2013

DOI:https://doi.org/10.1103/PhysRevA.88.033425

©2013 American Physical Society

Authors & Affiliations

Arun Nanduri1,*, Ashley Donovan2, Tak-San Ho2, and Herschel Rabitz2

  • 1Department of Physics, Princeton University, Princeton, New Jersey 08544, USA
  • 2Department of Chemistry, Princeton University, Princeton, New Jersey 08544, USA

  • *ananduri@princeton.edu

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Vol. 88, Iss. 3 — September 2013

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