NONLINEAR OPTICAL PHENOMENA

Resonance enhancement of nonlinear photoluminescence in gallium selenide and related compounds

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© 2012 Kvantovaya Elektronika and Turpion Ltd
, , Citation Ch Angermann et al 2012 Quantum Electron. 42 457 DOI 10.1070/QE2012v042n05ABEH014729

1063-7818/42/5/457

Abstract

Maker fringe experiments on the layered chalcogenide semiconductor gallium selenide (GaSe) with weak cw diode lasers are presented. It is demonstrated that nonlinear photoluminescence emitted by this material and by the similar compound GaSe0.9S0.1 under illumination with a 632.8-nm He — Ne laser shows very strong resonance enhancement upon heating when the absorption edge and exciton levels are shifted towards the laser line. The photoluminescence appears to be strongest when the energy level of the direct exciton, which emits it, is resonant with the photon energy of the laser. The previously observed enhancement of the photoluminescence by electric fields is interpreted in this context.

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10.1070/QE2012v042n05ABEH014729