透過您的圖書館登入
IP:52.14.224.197
  • 學位論文

利用碳奈米點表面電漿控制隨機雷射

Manipulation of Random Lasers Assisted by Plasmonic Carbon Nanodots

指導教授 : 陳永芳
若您是本文的作者,可授權文章由華藝線上圖書館中協助推廣。

摘要


碳奈米點(或是碳量子點)在近幾年成為熱門的研究材料,並且在生物以及光伏領域等取得廣泛的應用。雷射是生活中隨處可見的重要光電元件,然而迄今仍然缺乏碳量子點在雷射方面重要的應用。因此,在這篇論文中,我們藉由碳奈米點在2015年被發現的表面電漿性質的輔助,產生可以控制的隨機雷射訊號。蒐集燃燒蠟燭灰並分離產生的碳奈米點具有類似石墨烯的sp2鍵結結構,將少量的碳奈米點隨機裝飾在氮化鎵奈米柱的表面,藉此增強了氮化鎵的紫外輻射並產生了具有同調性的隨機雷射的訊號。除此之外,我們藉由改變碳奈米點的數量實現了雷射光學回饋以及雷射閾值的可調控性。這些可調控性對於光電元件的應用上非常重要。這個研究成果,不僅提供了利用表面電漿快速且簡單的控制隨機雷射的方法,也讓碳奈米點找到了在光電領域當中更廣泛的應用方法。

並列摘要


Carbon nanodots emerge as popular materials in various research fields, including biological and photovoltaic areas, while there lacks significant reports related to their applications in laser devices, which play a significant role in our daily life. In this work, we demonstrate the first controllable random laser assisted by the surface plasmon effect of carbon nanodots. Briefly, carbon nanodots derived from candle soot are randomly deposited on the surface of gallium nitride (GaN) nanorods to enhance the ultraviolet fluorescence of GaN and generate plasmonically enhanced random laser action with coherent feedback. Furthermore, potentially useful functionalities of tunable lasing threshold and controllable optical modes are achieved by adjusting the numbers of carbon nanodots, enabling for optical communication and identification technologies. In addition to providing an efficient alternative for plasmonically enahnced random laser devices with simple fabrication and low cost, our work also paves a useful route for the application of environmentally friendly carbon nanodots in optoelectronic devices.

參考文獻


2. Liao, Y. M.; Lai, Y. C.; Perumal, P.; Liao, W. C.; Chang, C. Y.; Liao, C. S.; Lin, S. Y.; Chen, Y. F., Highly Stretchable Label‐like Random Laser on Universal Substrates. Adv. Mater. Tech. 2016, 1.
1. Sun, T.-M.; Wang, C.-S.; Liao, C.-S.; Lin, S.-Y.; Perumal, P.; Chiang, C.-W.; Chen, Y.-F., Stretchable Random Lasers with Tunable Coherent Loops. ACS Nano 2015, 9, 12436-12441.
3. Wang, C. S.; Nieh, C. H.; Lin, T. Y.; Chen, Y. F., Electrically Driven Random Laser Memory. Adv. Funct. Mater. 2015, 25, 4058-4063.
4. Redding, B.; Choma, M. A.; Cao, H., Speckle-free laser imaging using random laser illumination. Nature photonics 2012, 6, 355-359.
5. Polson, R. C.; Vardeny, Z. V., Random lasing in human tissues. Appl. Phys. Lett. 2004, 85, 1289-1291.

延伸閱讀