基于高分辨质谱的石油组学分析技术的研究进展

doi:10.3724/SP.J.1123.2015.01016

摘要/Abstract

摘要：

随着原油重质化、劣质化程度的加深以及环境保护对燃油清洁性要求的日趋严格,对石油组成进行分子水平详细表征具有重大的现实意义和经济价值。依赖于高分辨质谱技术平台的石油组学分析技术成为实现这一目标的有力工具。本文以高分辨质谱技术平台为切入点,对石油组学定性定量分析技术的最新进展进行回顾和总结,并对其发展前景进行展望。

关键词: 分子组成, 石油, 石油组学, 质谱

Abstract:

As the increase of the remaining reserves of the heavier/sourer crude oil and the requirement of the clean energy, it is significant to sufficiently characterize the molecular composition of the petroleum for the selection of the refining processes and the realization of the economic value of the crude oil. Petroleomics, which is based on the high-resolution mass spectrometry platform, is a powerful tool to achieve this goal. In this paper, the analytical technology applied in petroleomics and its most recent development are reviewed, and the perspective of petroleomics is also discussed.

Key words: mass spectrometry, molecular composition, petroleomics, petroleum

中图分类号:

O658

宋春侠, 刘颖荣, 刘泽龙, 王威, 田松柏. 基于高分辨质谱的石油组学分析技术的研究进展[J]. 色谱, 2015, 33(5): 488-493.

SONG Chunxia, LIU Yingrong, LIU Zelong, WANG Wei, TIAN Songbai. Recent development in petroleomics based on the high-resolution mass spectrometry[J]. Chinese Journal of Chromatography, 2015, 33(5): 488-493.

参考文献

[1] Marshall A G, Rodgers R P. Acc Chem Res, 2004, 37(1): 53

[2] Rodgers R P, Schaub T M, Marshall A G. Anal Chem, 2005, 77(1): 20A

[3] Rodgers R P, McKenna A M. Anal Chem, 2011, 83(12): 4665

[4] Marshall A G, Rodgers R P. Proc Natl Acad Sci USA, 2008, 105(47): 18090

[5] Japan Petroleum Energy Center. The 4th Euro-Japan Conference for Petroleum Technology. (2011-08-31). http://www.pecj.or.jp/japanese/overseas/conference/pdf/conference08

[6] Song J Y, Cheng L. Contemporary Chemical Industry (宋锦玉, 成立. 当代化工), 2014, 43(8): 1498

[7] Panda S K, Andersson J T, Schrader W. Anal Bioanal Chem, 2007, 389(5): 1329

[8] Tang Y J, Wen Z G, Hou D J. Journal of Oil and Gas Technology (唐友军, 文志刚, 侯读杰. 石油天然气学报), 2006, 28(3): 23

[9] Van Geem K M, Pyl S P, Reyniers M F, et al. J Chromatogr A, 2010, 1217(43): 6623

[10] Gao X B, Chang Z Y, Dai W, et al. Chinese Journal of Chromatography (高儇博, 常振阳, 代威, 等. 色谱), 2014, 32(10): 1058

[11] Shi Q, Zhao S Q, Xu C M, et al. Journal of Chinese Mass Spectrometry Society (史权, 赵锁奇, 徐春明, 等. 质谱学报), 2008, 29(6): 367

[12] Shi Q, Zhang Y, Xu C, et al. Scientia Sinica Chimica, 2014, 44(5): 694

[13] Hsu C S, Hendrickson C L, Rodgers R P, et al. J Mass Spectrom, 2011, 46(4): 337

[14] Schaub T M, Linden H B, Hendrickson C L, et al. Rapid Commun Mass Spectrom, 2004, 18(14): 1641

[15] Smith D F, Schaub T M, Rodgers R P, et al. Anal Chem, 2008, 80(19): 7379

[16] Linden H B, Gross J H. Rapid Commun Mass Spectrom, 2012, 26(3): 336

[17] Zhan D, Fenn J B. Int J Ion Mobility Spectrom, 2000, 194(2): 197

[18] Qian K, Robbins W K, Hughey C A, et al. Energy Fuels, 2001, 15(6): 1505

[19] Liu Y R, Liu Z L, Zhu X Y, et al. Journal of Chinese Mass Spectrometry Society (刘颖荣, 刘泽龙, 祝馨怡, 等. 质谱学报), 2008, 29: 54

[20] Panda S K, Andersson J T, Schrader W. Angew Chem Int Ed, 2009, 48(10): 1788

[21] Lobodin V V, Juyal P, McKenna A M, et al. Energy Fuels, 2014, 28(1): 447

[22] Fujii T. Mass Spectrom Rev, 2000, 19(3): 111

[23] Lobodin V V, Juyal P, McKenna A M, et al. Energy Fuels, 2014, 28(11): 6841

[24] Purcell J M, Hendrickson C L, Rodgers R P, et al. Anal Chem, 2006, 78(16): 5906

[25] Bae E, Na J G, Chung S H, et al. Energy Fuels, 2010, 24(4): 2563

[26] Cho Y, Ahmed A, Kim S. Anal Chem, 2013, 85(20): 9758

[27] Panda S K, Brockmann K J, Benter T, et al. Rapid Commun Mass Spectrom, 2011, 25(16): 2317

[28] Kim Y H, Kim S. J Am Soc Mass Spectrom, 2010, 21(3): 386

[29] Pereira T M C, Vanini G, Tose L V, et al. Fuel, 2014, 131: 49

[30] Wu C, Qian K, Nefliu M, et al. J Am Soc Mass Spectrom, 2010, 21(2): 261

[31] Rummel J L, McKenna A M, Marshall A G, et al. Rapid Commun Mass Spectrom, 2010, 24(6): 784

[32] Nyadong L, McKenna A M, Hendrickson C L, et al. Anal Chem, 2011, 83(5): 1616

[33] Du Z H, Zhang L, Liu S Y. Chinese Journal of Chromatography (杜振华, 张磊, 刘树业. 色谱), 2011, 29(4): 314

[34] Cao X L, Gong J D, Chen M X, et al. Chinese Journal of Chromatography (曹晓林, 巩佳第, 陈铭学, 等. 色谱), 2014, 32(11): 1181

[35] Smith E A, Lee Y J. Energy Fuels, 2010, 24(9): 5190

[36] Pomerantz A E, Mullins O C, Paul G, et al. Energy Fuels, 2011, 25(7): 3077

[37] Zhurov K O, Kozhinov A N, Tsybin Y O. Energy Fuels, 2013, 27(6): 2974

[38] Kozhinov A N, Zhurov K O, Tsybin Y O. Anal Chem, 2013, 85(13): 6437

[39] Becker C, Fernandez Lima F A, Russell D H. Spectroscopy, 2009, 24(4): 38

[40] Hertkorn N, Ruecker C, Meringer M, et al. Anal Bioanal Chem, 2007, 389(5): 1311

[41] Ruotolo B T, Tate C C, Russell D H. J Am Soc Mass Spectrom, 2004, 15(6): 870

[42] Sawyer H A, Marini J T, Stone E G, et al. J Am Soc Mass Spectrom, 2005, 16(6): 893

[43] Hoffmann W, Hofmann J, Pagel K. J Am Soc Mass Spectrom, 2014, 25(3): 471

[44] Ohshimo K, Komukai T, Moriyama R, et al. J Phys Chem A, 2014, 118(22): 3899

[45] Cossoul E, Hubert-Roux M, Sebban M, et al. Anal Chim Acta, 2015, 856: 46

[46] Barrere C, Selmi W, Hubert-Roux M, et al. Polym Chem, 2014, 5(11): 3576

[47] Becker C, Qian K, Russell D H. Anal Chem, 2008, 80(22): 8592

[48] Fernandez-Lima F A, Becker C, McKenna A M, et al. Anal Chem, 2009, 81(24): 9941

[49] Ahmed A, Cho Y J, No M, et al. Anal Chem, 2011, 83(1): 77

[50] Ahmed A, Cho Y, Giles K, et al. Anal Chem, 2014, 86(7): 3300

[51] Maire F, Neeson K, Denny R, et al. Anal Chem, 2013, 85(11): 5530

[52] Fasciotti M, Lalli P M, Klitzke C F, et al. Energy Fuels, 2013, 27(12): 7277

[53] Ponthus J, Riches E. Int J Ion Mobility Spectrom, 2013, 16(2): 95

[54] Fasciotti M, Lalli P M, Heerdt G, et al. Int J Ion Mobility Spectrom, 2013, 16(2): 117

[55] Zhou Y, Zhang K, Yuan H M, et al. Chinese Journal of Chromatography (周愿, 张珅, 袁辉明, 等. 色谱), 2014, 32(4): 355

[56] Du J H, Liu X, Xu X P. Chinese Journal of Chromatography (杜晶辉, 刘旭, 徐小平. 色谱), 2014, 32(1): 7

[57] Kim S, Rodgers R P, Blakney G T, et al. J Am Soc Mass Spectrom, 2009, 20(2): 263

[58] Haapala M, Purcell J M, Saarela V, et al. Anal Chem, 2009, 81(7): 2799

[59] Jjunju F P M, Li A, Badu-Tawiah A, et al. Analyst, 2013, 138(13): 3740

[60] Gaspar A, Zellermann E, Lababidi S, et al. Anal Chem, 2012, 84(12): 5257