Skip to main content
SpringerLink
Log in

Influence of temperature on the speciation of radionuclides sorbed onto rocks from the Nizhnekansky massif

  • Published:
Radiochemistry Aims and scope

Abstract

The influence of temperature on speciation of actinides (Pu, Am) and some fission products (Cs, Sr), sorbed from simulated groundwater onto rocks from the Nizhnekansky massif (gneiss, dolerite) under anaerobic conditions at 20 and 90°С, was studied by sequential extraction. An increase in the contact temperature leads to an increase in the radionuclide uptake percentage and, in some cases, in the content of tightly fixed forms. The radionuclide species undergo redistribution with time.

This is a preview of subscription content, log in via an institution to check access.

Access this article

Log in via an institution

Price excludes VAT (USA)
Tax calculation will be finalised during checkout.

Instant access to the full article PDF.

Institutional subscriptions

Similar content being viewed by others

References

  1. Bacon, J.R. and Davidson, C.M., Analyst, 2008, vol. 133, pp. 25–46.

    Article  CAS  Google Scholar 

  2. Tessier, A., Campbell, P.G.C., and Bisson, M., Anal. Chem., 1979, vol. 51, no. 7, pp. 844–851.

    Article  CAS  Google Scholar 

  3. Goryachenkova, T.A., Kazinskaya, I.E., Clark, S.B., et al., Radiochemistry, 2005, vol. 47, no. 6, pp. 599–604.

    Article  CAS  Google Scholar 

  4. Novikov, A.P., Goryachenkova, T.A., Kalmykov, S.N., et al., Radiochemistry, 2009, vol. 51, no. 6, pp. 649–653.

    Article  CAS  Google Scholar 

  5. Vlasova, I.E., Kalmykov, St.N., Konevnik, Yu.V., et al., Radiat. Meas., 2008, vol. 43, pp. S303–S308.

    Article  CAS  Google Scholar 

  6. Sabodina, M.N., Zakharova, E.V., Mironenko, M.V., et al., Radiochemistry, 2009, vol. 51, no. 4, pp. 422–424.

    Article  CAS  Google Scholar 

  7. Lujaniene, G., Benes, P., Stamberg, K., et al., J. Environ. Radioact., 2012, vol. 108, pp. 41–49.

    Article  CAS  Google Scholar 

  8. Walton, F.B., Melnyk, T.W., Ross, J.P.M., and Skeet, A.M.M., Am. Chem. Soc. Symp. Ser., 1984, vol. 246, pp. 45–66.

    CAS  Google Scholar 

  9. Fujikawa, Y. and Fukui, M., J. Contam. Hydrol., 1991, vol. 8, pp. 177–195.

    Article  CAS  Google Scholar 

  10. Anderson, E.B., Rogozin, Yu.M., Smirnova, E.A., et al., Radiochemistry, 2007, vol. 49, no. 3, pp. 305–312.

    Article  CAS  Google Scholar 

  11. Römer, J., Kienzler, B., and Schild, D., in Proc. 1st Annual Workshop, 6th ECFP-FUNMIG IP,Saclay (France), 2005, pp. 132–136.

    Google Scholar 

  12. Puukko, E., Puhakka, E., Lindberg, A., et al., in Proc. 1st Annual Workshop, 6th ECFP-FUNMIG IP,Saclay (France), 2005, pp. 80–85.

    Google Scholar 

  13. Konevni., Yu.V., Zakharova, E.V., Martynov, K.V., et al., Radiochemistry, 2017, vol. 59, no. 3, pp. 274–279.

    Google Scholar 

  14. Kolotov, V.P., Grozdov, D.S., Dogadkin, N.N., et al., J. Anal. Chem., 2015, vol. 70, no. 3, pp. 287–291.

    Article  CAS  Google Scholar 

  15. Subbotin, S.B., Dubasov, Yu.V., Korovina, O.Yu., and Smirnova, E.A., Radiochemistry, 2014, vol. 56, no. 5, pp. 560–564.

    Article  CAS  Google Scholar 

  16. Lavrinovich, E.A., Goryachenkova, T.A., Abramova, A.V., and Novikov, A.P., Radiochemistry, 2014, vol. 56, no. 2, pp. 216–221.

    Article  CAS  Google Scholar 

  17. Bates, J.K., Bradley, J.P., Teetsov, A., et al., Science, 1992, vol. 256, pp. 649–651.

    Article  CAS  Google Scholar 

  18. Kulyak., Yu.M., Trofimov, T.I., Malikov, D.A., et al., Radiochemistry, 2010, vol. 52, no. 4, pp. 366–370.

    Article  Google Scholar 

  19. Trofimov, T.I., Kulyako, Yu.M., Perevalov, S.A., et al., Radiochemistry, 2009, vol. 51, no. 1, pp. 18–25.

    Article  CAS  Google Scholar 

Download references

Author information

Authors and Affiliations

  1. Frumkin Institute of Physical Chemistry and Electrochemistry, Russian Academy of Sciences, Leninskii pr. 31, korp. 4, Moscow, 119071, Russia

    Yu. V. Konevnik, E. V. Zakharova, K. V. Martynov & A. A. Shiryaev

Authors
  1. Yu. V. Konevnik
    View author publications

    You can also search for this author in PubMed Google Scholar

  2. E. V. Zakharova
    View author publications

    You can also search for this author in PubMed Google Scholar

  3. K. V. Martynov
    View author publications

    You can also search for this author in PubMed Google Scholar

  4. A. A. Shiryaev
    View author publications

    You can also search for this author in PubMed Google Scholar

Corresponding author

Correspondence to Yu. V. Konevnik.

Additional information

Original Russian Text © Yu.V. Konevnik, E.V. Zakharova, K.V. Martynov, A.A. Shiryaev, 2017, published in Radiokhimiya, 2017, Vol. 59, No. 3, pp. 280–284.

Rights and permissions

Reprints and permissions

About this article

Check for updates. Verify currency and authenticity via CrossMark

Cite this article

Konevnik, Y.V., Zakharova, E.V., Martynov, K.V. et al. Influence of temperature on the speciation of radionuclides sorbed onto rocks from the Nizhnekansky massif. Radiochemistry 59, 320–325 (2017). https://doi.org/10.1134/S1066362217020171

Download citation

  • Received:

  • Published:

  • Issue Date:

  • DOI: https://doi.org/10.1134/S1066362217020171

Keywords

Search

Navigation