Frustration Driven Lattice Distortion: An NMR Investigation of Y2Mo2O7

Amit Keren and Jason S. Gardner
Phys. Rev. Lett. 87, 177201 – Published 3 October 2001
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Abstract

We have investigated the 89Y NMR spectrum and spin lattice relaxation, T1, in the magnetically frustrated pyrochlore Y2Mo2O7. We find that upon cooling the spectrum shifts, and broadens asymmetrically. A detailed examination of the low T spectrum reveals that it is constructed from multiple peaks, each shifted by a different amount. We argue that this spectrum is due to discrete lattice distortions and speculate that these distortions relieve the frustration and reduce the system’s energy.

  • Received 25 May 2001

DOI:https://doi.org/10.1103/PhysRevLett.87.177201

©2001 American Physical Society

Authors & Affiliations

Amit Keren1 and Jason S. Gardner2

  • 1Department of Physics, Technion–Israel Institute of Technology, Haifa 32000, Israel
  • 2NRC Canada, NPMR, Chalk River Laboratories, Chalk River, Ontario, Canada K0J 1J0

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Vol. 87, Iss. 17 — 22 October 2001

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