Abstract
The dephasing of excitonic localized states is investigated in mixed crystals at 2 K with low intensity femtosecond optical pulses. We observe a fast relaxation process which is first reported here. It is shown to be related to the creation of localized biexcitons via the exciton-biexciton transitions which act as an additional dephasing mechanism with a time constant of 700 fs. The coherence between excitonic and biexcitonic states, which manifests by 800 fs period beats, is studied in detail. A simple model is presented which describes both the fast initial decay and the beating behavior.
- Received 1 March 1993
DOI:https://doi.org/10.1103/PhysRevLett.71.1820
©1993 American Physical Society