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Optical Detection of Long Electron Spin Transport Lengths in a Monolayer Semiconductor

L. Ren (任磊), L. Lombez, C. Robert, D. Beret, D. Lagarde, B. Urbaszek, P. Renucci, T. Taniguchi, K. Watanabe, S. A. Crooker, and X. Marie
Phys. Rev. Lett. 129, 027402 – Published 5 July 2022
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Abstract

Using a spatially resolved optical pump-probe experiment, we measure the lateral transport of spin-valley polarized electrons over very long distances (tens of micrometers) in a single WSe2 monolayer. By locally pumping the Fermi sea of 2D electrons to a high degree of spin-valley polarization (up to 75%) using circularly polarized light, the lateral diffusion of the electron polarization can be mapped out via the photoluminescence induced by a spatially separated and linearly polarized probe laser. Up to 25% spin-valley polarization is observed at pump-probe separations up to 20μm. Characteristic spin-valley diffusion lengths of 18±3μm are revealed at low temperatures. The dependence on temperature, pump helicity, pump intensity, and electron density highlight the key roles played by spin relaxation time and pumping efficiency on polarized electron transport in monolayer semiconductors possessing spin-valley locking.

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  • Received 27 January 2022
  • Accepted 18 May 2022

DOI:https://doi.org/10.1103/PhysRevLett.129.027402

© 2022 American Physical Society

Physics Subject Headings (PhySH)

Condensed Matter, Materials & Applied Physics

Authors & Affiliations

L. Ren (任磊)1,*, L. Lombez1,*, C. Robert1,*,†, D. Beret1, D. Lagarde1, B. Urbaszek1, P. Renucci1, T. Taniguchi2, K. Watanabe3, S. A. Crooker4, and X. Marie1,‡

  • 1Université de Toulouse, INSA-CNRS-UPS, LPCNO, 135 Av. Rangueil, 31077 Toulouse, France
  • 2International Center for Materials Nanoarchitectonics, National Institute for Materials Science, 1-1 Namiki, Tsukuba 305-00044, Japan
  • 3Research Center for Functional Materials, National Institute for Materials Science, 1-1 Namiki, Tsukuba 305-00044, Japan
  • 4National High Magnetic Field Laboratory, Los Alamos National Laboratory, Los Alamos, New Mexico 87545, USA

  • *These authors contributed equally to this work.
  • Corresponding author. cerobert@insa-toulouse.fr
  • Corresponding author. xavier.marie@insa-toulouse.fr

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Issue

Vol. 129, Iss. 2 — 8 July 2022

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