Abstract
The nonlinear optical response to high fields is absolutely measured for the noble gas atoms He, Ne, Ar, Kr, and Xe. We find that the response is quadratic in the laser field magnitude up to the ionization threshold of each gas. Its size and quadratic dependence are well predicted by a Kramers-Kronig analysis employing known ionization probabilities, and the results are consistent with calculations using the time-dependent Schrödinger equation.
- Received 20 February 2012
DOI:https://doi.org/10.1103/PhysRevLett.109.113904
© 2012 American Physical Society