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Extended fluctuation-dissipation theorem for soft matter in stationary flow

Thomas Speck and Udo Seifert
Phys. Rev. E 79, 040102(R) – Published 22 April 2009
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Abstract

For soft matter systems strongly driven by stationary flow, we discuss an extended fluctuation-dissipation theorem (FDT). Beyond the linear-response regime, the FDT for the stress acquires an additional contribution involving the observable that is conjugate to the strain rate with respect to the dissipation function. This extended FDT is evaluated both analytically for Rouse polymers and in numerical simulations for colloidal suspensions. More generally, our results suggest an extension of Onsager’s regression principle to nonequilibrium steady states.

    • Received 28 January 2009

    DOI:https://doi.org/10.1103/PhysRevE.79.040102

    ©2009 American Physical Society

    Authors & Affiliations

    Thomas Speck* and Udo Seifert

    • II. Institut für Theoretische Physik, Universität Stuttgart, Pfaffenwaldring 57, 70550 Stuttgart, Germany

    • *Present address: Department of Chemistry, University of California, Berkeley, CA 94720, USA.

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    Issue

    Vol. 79, Iss. 4 — April 2009

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