Spontaneous fission modes and lifetimes of superheavy elements in the nuclear density functional theory

A. Staszczak, A. Baran, and W. Nazarewicz
Phys. Rev. C 87, 024320 – Published 27 February 2013

Abstract

Background: The reactions with the neutron-rich 48Ca beam and actinide targets resulted in the detection of new superheavy (SH) nuclides with Z=104118. The unambiguous identification of the new isotopes, however, still poses a problem because their α-decay chains terminate by spontaneous fission (SF) before reaching the known region of the nuclear chart. The understanding of the competition between α-decay and SF channels in SH nuclei is, therefore, of crucial importance for our ability to map the SH region and to assess its extent.

Purpose: We perform self-consistent calculations of the competing decay modes of even-even SH isotopes with 108Z126 and 148N188.

Methods: We use the state-of-the-art computational framework based on self-consistent symmetry-unrestricted nuclear density functional theory capable of describing the competition between nuclear attraction and electrostatic repulsion. We apply the SkM* Skyrme energy density functional. The collective mass tensor of the fissioning superfluid nucleus is computed by means of the cranking approximation to the adiabatic time-dependent Hartree-Fock-Bogoliubov (HFB) approach. This paper constitutes a systematic self-consistent study of spontaneous fission in the SH region, carried out at a full HFB level, that simultaneously takes into account both triaxiality and reflection asymmetry.

Results: Breaking axial symmetry and parity turns out to be crucial for a realistic estimate of collective action; it results in lowering SF lifetimes by more than 7 orders of magnitude in some cases. We predict two competing SF modes: reflection symmetric modes and reflection asymmetric modes.

Conclusions: The shortest-lived SH isotopes decay by SF; they are expected to lie in a narrow corridor formed by 280Hs, 284Fl, and 118284Uuo that separates the regions of SH nuclei synthesized in “cold-fusion” and “hot-fusion” reactions. The region of long-lived SH nuclei is expected to be centered on 294Ds with a total half-life of 1.5days. Our survey provides a solid benchmark for the future improvements of self-consistent SF calculations in the region of SH nuclei.

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  • Received 26 July 2012

DOI:https://doi.org/10.1103/PhysRevC.87.024320

©2013 American Physical Society

Authors & Affiliations

A. Staszczak1,2,3, A. Baran1,2,3, and W. Nazarewicz2,3,4

  • 1Institute of Physics, Maria Curie-Skłodowska University, pl. M. Curie-Skłodowskiej 1, 20-031 Lublin, Poland
  • 2Department of Physics and Astronomy, University of Tennessee Knoxville, Tennessee 37996, USA
  • 3Oak Ridge National Laboratory, P.O. Box 2008, Oak Ridge, Tennessee 37831, USA
  • 4Theoretical Physics, University of Warsaw, ul. Hoża 69, 00-681 Warsaw, Poland

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Issue

Vol. 87, Iss. 2 — February 2013

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