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Magnetic states and spin-glass properties in Bi0.67Ca0.33MnO3: Macroscopic ac measurements and neutron scattering

Maud Giot, Alain Pautrat, Gilles André, Damien Saurel, Maryvonne Hervieu, and Juan Rodriguez-Carvajal
Phys. Rev. B 77, 134445 – Published 29 April 2008

Abstract

We report on the magnetic properties of the manganite Bi1xCaxMnO3 (x=0.33) at low temperature. The analysis of the field expansion of the ac susceptibility and the observation of aging properties make clear that a spin-glass phase appears below T=39K in the presence of magnetic order. Neutron scattering shows both magnetic Bragg scattering and magnetic diffusion at small angles and confirms this coexistence. In contrast to Pr1xCaxMnO3 (x=0.30.33), which exhibits a mesoscopic phase separation responsible for a field driven percolation, the glassy and short range ferromagnetic order observed here does not cause a colossal magnetoresistance.

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  • Received 1 February 2008

DOI:https://doi.org/10.1103/PhysRevB.77.134445

©2008 American Physical Society

Authors & Affiliations

Maud Giot1,2,*, Alain Pautrat1, Gilles André2, Damien Saurel3, Maryvonne Hervieu1, and Juan Rodriguez-Carvajal4

  • 1Laboratoire CRISMAT, UMR 6508 du CNRS, ENSICAEN et Université de Caen, 6 Boulevard Maréchal Juin, F-14050 Caen 4, France
  • 2Laboratoire Léon Brillouin, CEA Saclay, 91191 Gif/Yvette, France
  • 3Nanoscale Superconductivity and Magnetism and Pulsed Fields Group, Institute for Nanoscale Physics and Chemistry (INPAC), K. U. Leuven, Celestijnenlaan 200 D, 3001 Leuven, Belgium
  • 4Institut Laue-Langevin, 6, rue Jules Horowitz, Boîte Postate 156, 38042 Grenoble Cedex 9, France

  • *Also at SPMS, UMR CNRS 8580, Ecole Centrale de Paris, 92295 Châtenay-Malabry, France and DEN/DMN/SRMA/LA2M, CEA Saclay, 91191 Gif-sur-Yvette, France.

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Issue

Vol. 77, Iss. 13 — 1 April 2008

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