Elastic-neutron-scattering study of the devil’s-staircase behavior in deuterated betaine calcium chloride dihydrate

A. Almeida, M. R. Chaves, J. M. Kiat, J. Schneck, W. Schwarz, J. C. Tolédano, J. L. Ribeiro, A. Klöpperpieper, H. E. Müser, and J. Albers
Phys. Rev. B 45, 9576 – Published 1 May 1992
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Abstract

An elastic-neutron-scattering study of partially deuterated dihydrate betaine calcium chloride (D-BCCD) is reported. We obtain direct diffraction evidence for the occurrence of a commensurate phase with wave vector qc*=(2/9)c* and for the absence of modulation of the lowest-temperature phase. The existence of another incommensurate phase adjacent to the δ=2/9 commensurate phase is pointed out and some indications of the existence of the δ=2/7 commensurate phase are described. Diffraction data relative to the temperature dependence of the modulation wavelength and to its amplitude are discussed in the light of the present controversy relative to the theoretical scheme relevant to BCCD.

  • Received 5 August 1991

DOI:https://doi.org/10.1103/PhysRevB.45.9576

©1992 American Physical Society

Authors & Affiliations

A. Almeida and M. R. Chaves

  • Centro de Física da Universidade do Porto, Instituto Nacional De Investigação Cientifica (INIC), Faculdade de Ciências, Universidade do Porto, 4000 Porto, Portugal

J. M. Kiat

  • Laboratoire Léon Brillouin, Centre d’Études Nucléaires de Saclay, 91191 Gif-sur-Yvette CEDEX, France
  • Ecole Centrale, Chemin des Vignes, 92290 Chatenay, Malabry, France

J. Schneck

  • Centre National d’Études des Télécommunications, Bagneux 92220, France

W. Schwarz

  • Laboratoire Léon Brillouin, Centre d’Études Nucléaires de Saclay, 91191 Gif-sur-Yvette CEDEX, France
  • Institut für Experimental Physik, Universität of Vienna, Austria

J. C. Tolédano

  • Centre National d’Études des Télécommunications, Bagneux 92220, France

J. L. Ribeiro

  • Centro de Física da Universidade do Porto (INIC), Faculdade de Ciências, Universidade do Porto, 4000 Porto, Portugal

A. Klöpperpieper, H. E. Müser, and J. Albers

  • Fachbereich Physik, Universität des Saarlandes, 6000 Saarbrücken, Germany

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Issue

Vol. 45, Iss. 17 — 1 May 1992

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