Carrier Diffusion in GaN: A Cathodoluminescence Study. I. Temperature-Dependent Generation Volume

Uwe Jahn, Vladimir M. Kaganer, Karl K. Sabelfeld, Anastasya E. Kireeva, Jonas Lähnemann, Carsten Pfüller, Timur Flissikowski, Caroline Chèze, Klaus Biermann, Raffaella Calarco, and Oliver Brandt
Phys. Rev. Applied 17, 024017 – Published 7 February 2022

Abstract

The determination of the carrier diffusion length of semiconductors such as GaN and GaAs by cathodoluminescence imaging requires accurate knowledge about the spatial distribution of generated carriers. To obtain the lateral distribution of generated carriers for sample temperatures between 10 and 300 K, we utilize cathodoluminescence intensity profiles measured across single quantum wells embedded in thick GaN and GaAs layers. Thin (Al,Ga)N and (Al,Ga)As barriers respectively prevent carriers diffusing in the GaN and GaAs layers to reach the well, which would broaden the profiles. The experimental cathodoluminescence profiles are found to be systematically wider than the energy loss distributions calculated by means of the Monte Carlo program casino, with the width monotonically increasing with decreasing temperature. This effect is observed for both GaN and GaAs and becomes more pronounced for higher acceleration voltages. We discuss this phenomenon in terms of both the electron-phonon interaction controlling the energy relaxation of hot carriers and the shape of the initial carrier distribution. Finally, we present a phenomenological approach to simulate the carrier generation volume that can be used for the investigation of the temperature dependence of carrier diffusion.

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  • Received 4 December 2020
  • Revised 24 November 2021
  • Accepted 18 January 2022

DOI:https://doi.org/10.1103/PhysRevApplied.17.024017

© 2022 American Physical Society

Physics Subject Headings (PhySH)

Condensed Matter, Materials & Applied Physics

Authors & Affiliations

Uwe Jahn1, Vladimir M. Kaganer1, Karl K. Sabelfeld2, Anastasya E. Kireeva2, Jonas Lähnemann1,*, Carsten Pfüller1, Timur Flissikowski1, Caroline Chèze1, Klaus Biermann1, Raffaella Calarco1,‡, and Oliver Brandt1,†

  • 1Paul-Drude-Institut für Festkörperelektronik, Leibniz-Institut im Forschungsverbund Berlin e.V., Hausvogteiplatz 5–7, Berlin 10117, Germany
  • 2Institute of Computational Mathematics and Mathematical Geophysics, Russian Academy of Sciences, Lavrentiev Prosp. 6, Novosibirsk 630090, Russia

  • *laehnemann@pdi-berlin.de
  • brandt@pdi-berlin.de
  • Present address: Istituto per la Microelettronica e Microsistemi, Consiglio Nazionale delle Ricerche, via del Fosso del Cavaliere 100, 00133 Roma, Italy.

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Vol. 17, Iss. 2 — February 2022

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