Positron scattering from pyrazine

D. Edwards, D. Stevens, Z. Cheong, V. Graves, J. D. Gorfinkiel, F. Blanco, G. Garcia, M. J. Brunger, R. D. White, and J. P. Sullivan
Phys. Rev. A 104, 042807 – Published 12 October 2021

Abstract

The present paper provides a joint experimental and theoretical study of positron scattering from pyrazine. Experimental data were measured employing a low-energy positron beamline, and covered an energy range from 1 to 79 eV. Cross sections were measured for total scattering, total elastic scattering, positronium formation, direct ionization, and the sum of the total discrete electronic-state excitation processes. In addition, measured total electronic excitation cross sections for the individual 11B3u, 11B2u, 11B1u, and 21B2u states are also reported. Finally, experimental elastic differential cross sections (DCSs), here in the energy range 120 eV, are also presented. Results from two theoretical approaches are given: the R-matrix approach and the independent atom method with screening corrected additivity rule and interference terms. Where a comparison between our experimental and theoretical results could be made, the level of accord varied from being quite good to marginal depending on the actual scattering process under consideration. Last, a comparison between the present elastic DCS results and those from our earlier study on positron scattering from pyrimidine [Palihawadana et al., Phys. Rev. A 88, 012717 (2013)] showed a somewhat unexpected level of agreement.

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  • Received 11 July 2021
  • Accepted 24 September 2021

DOI:https://doi.org/10.1103/PhysRevA.104.042807

©2021 American Physical Society

Physics Subject Headings (PhySH)

Atomic, Molecular & Optical

Authors & Affiliations

D. Edwards1, D. Stevens1, Z. Cheong1, V. Graves2, J. D. Gorfinkiel2, F. Blanco3, G. Garcia4, M. J. Brunger5,6, R. D. White7, and J. P. Sullivan1

  • 1Laser Physics Centre, Research School of Physics, Australian National University, 2601 Canberra, Australia
  • 2School of Physical Sciences, The Open University, Walton Hall, MK7 6AA Milton Keynes, United Kingdom
  • 3Departamento de Estructura de la Materia, Fisica Termica y Electronica e IPARCOS, Universidad Complutense de Madrid, 28040 Madrid, Spain
  • 4Instituto de Fısica Fundamental, Consejo Superior de Investigaciones Cientificas, Serrano 113-bis, 28006 Madrid, Spain
  • 5College of Science and Engineering, Flinders University, Adelaide, 5042 South Australia, Australia
  • 6Department of Actuarial Science and Applied Statistics, Faculty of Business and Management, UCSI University, Kuala Lumpur 56000, Malaysia
  • 7College of Science and Engineering, James Cook University, Townsville, 4810 Queensland, Australia

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Issue

Vol. 104, Iss. 4 — October 2021

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