Abstract
The newly developed technique of polarization pulse shaping is applied to the control of two-photon absorption in atomic rubidium. This technique enables the manipulation of the transient vector properties of a light matter interaction. We establish that control can be exerted on the angular distribution of the final state, and demonstrate the ability to control the final state population of a nearly degenerate system, as well as to perform -state resolved spectroscopy.
- Received 7 October 2003
DOI:https://doi.org/10.1103/PhysRevLett.92.103003
©2004 American Physical Society