Singlet Ground State of the Quantum Antiferromagnet Ba3CuSb2O9

J. A. Quilliam, F. Bert, E. Kermarrec, C. Payen, C. Guillot-Deudon, P. Bonville, C. Baines, H. Luetkens, and P. Mendels
Phys. Rev. Lett. 109, 117203 – Published 11 September 2012
PDFHTMLExport Citation

Abstract

We present local probe results on the honeycomb lattice antiferromagnet Ba3CuSb2O9. Muon spin relaxation measurements in a zero field down to 20 mK show unequivocally that there is a total absence of spin freezing in the ground state. Sb NMR measurements allow us to track the intrinsic susceptibility of the lattice, which shows a maximum at around 55 K and drops to zero in the low-temperature limit. The spin-lattice relaxation rate shows two characteristic energy scales, including a field-dependent crossover to exponential low-temperature behavior, implying gapped magnetic excitations.

  • Figure
  • Figure
  • Figure
  • Figure
  • Received 8 June 2012

DOI:https://doi.org/10.1103/PhysRevLett.109.117203

© 2012 American Physical Society

Authors & Affiliations

J. A. Quilliam1, F. Bert1, E. Kermarrec1, C. Payen2, C. Guillot-Deudon2, P. Bonville3, C. Baines4, H. Luetkens4, and P. Mendels1,5

  • 1Laboratoire de Physique des Solides, Université Paris-Sud 11, UMR CNRS 8502, 91405 Orsay, France
  • 2Institut des Matériaux Jean Rouxel, UMR 6502 Université de Nantes, CNRS, 2 rue de la Houssinière, BP 32229, 44322 Nantes Cedex 3, France
  • 3Service de Physique de lÉtat Condensé, CEA-CNRS, CE-Saclay, F-91191 Gif-Sur-Yvette, France
  • 4Laboratory for Muon Spin Spectroscopy, Paul Scherrer Institute, CH-5232 Villigen PSI, Switzerland
  • 5Institut Universitaire de France, 103 Boulevard Saint-Michel, F-75005 Paris, France

Article Text (Subscription Required)

Click to Expand

Supplemental Material (Subscription Required)

Click to Expand

References (Subscription Required)

Click to Expand
Issue

Vol. 109, Iss. 11 — 14 September 2012

Reuse & Permissions
Access Options
Author publication services for translation and copyediting assistance advertisement

Authorization Required


×
×

Images

×

Sign up to receive regular email alerts from Physical Review Letters

Log In

Cancel
×

Search


Article Lookup

Paste a citation or DOI

Enter a citation
×