Phase-ordering kinetics in the Allen-Cahn (Model A) class: Universal aspects elucidated by electrically induced transition in liquid crystals

Renan A. L. Almeida and Kazumasa A. Takeuchi
Phys. Rev. E 104, 054103 – Published 5 November 2021
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Abstract

The two-dimensional (2D) Ising model is the statistical physics textbook example for phase transitions and their kinetics. Quenched through the Curie point with Glauber rates, the late-time description of the ferromagnetic domain coarsening finds its place at the scalar sector of the Allen-Cahn (or Model A) class, which encompasses phase-ordering kinetics endowed with a nonconserved order parameter. Resisting exact results sought for theoreticians since Lifshitz's first account in 1962, the central quantities of 2D Model A—most scaling exponents and correlation functions—remain known up to approximate theories whose disparate outcomes urge experimental assessment. Here we perform such assessment based on a comprehensive study of the coarsening of 2D twisted nematic liquid crystals whose kinetics is induced by a superfast electrical switching from a spatiotemporally chaotic (disordered) state to a two-phase concurrent, equilibrium one. Tracking the dynamics via optical microscopy, we first show the sharp evidence of well-established Model A aspects, such as the dynamic exponent z=2 and the dynamic scaling hypothesis, to then move forward. We confirm the Bray-Humayun theory for Porod's regime describing intradomain length scales of the two-point spatial correlators and show that their nontrivial decay beyond the Porod's scale can be captured in a free-from-parameter fashion by Gaussian theories, namely the Ohta-Jasnow-Kawasaki (OJK) and Mazenko theories. Regarding time-related statistics, we corroborate the aging hypothesis in Model A systems, which includes the collapse of two-time correlators into a master curve whose format is, actually, best accounted for by a solution of the local scaling invariance theory: the same solution that fits the 2D nonconserved Ising model correlator along with the Fisher-Huse conjecture. We also suggest the true value for the local persistence exponent in Model A class, in disfavor of the exact outcome for the diffusion and OJK equations. Finally, we observe a fractal morphology for persistence clusters and extract their universal dimension. Given its accuracy and possibilities, this experimental setup may work as a prototype to address further universality issues in the realm of nonequilibrium systems.

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  • Received 20 July 2021
  • Accepted 27 September 2021

DOI:https://doi.org/10.1103/PhysRevE.104.054103

©2021 American Physical Society

Physics Subject Headings (PhySH)

Statistical Physics & ThermodynamicsPolymers & Soft Matter

Authors & Affiliations

Renan A. L. Almeida1,2,3,* and Kazumasa A. Takeuchi3,†

  • 1Department of Physics, Tokyo Institute of Technology, 2-12-1 Ookayama, Meguro-ku, Tokyo 152-8551, Japan
  • 2Departmento de Física, Universidade Federal de Viçosa, 36570-900 Viçosa, MG, Brazil
  • 3Department of Physics, The University of Tokyo, 7-3-1 Hongo, Bunkyo-ku, Tokyo 113-0033, Japan

  • *renan.lisboaufv@gmail.com
  • kat@kaztake.org

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Issue

Vol. 104, Iss. 5 — November 2021

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