Fission of Pu240 with 14.8-MeV neutrons

D. R. Nethaway, A. L. Prindle, William A. Myers, W. C. Fuqua, and M. V. Kantelo
Phys. Rev. C 16, 1907 – Published 1 November 1977
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Abstract

We have measured the mass-yield distribution from the fission of Pu240 induced by 14.8-MeV neutrons. Seventy-five fission products from Ni66 to Er169 were detected. From these measurements we obtained the total chain yields for 49 mass numbers and constructed the mass-yield curve. Absolute fission yields were obtained by using the U238(n,f) monitor reaction. The total yield determined from each half of the mass-yield curve is 0.984. From the agreement in these two methods we conclude that our yield determination is accurate to approximately 4%. The peak-to-valley ratio is 5.5, a significantly larger value than the ratio of 4.1 found for 14.8-MeV neutron fission of Pu239. This difference agrees with the trend noted previously for 14.8-MeV neutron fission of uranium isotopes. A number of independent fission yields were measured. Values of Zp inferred from these yields agree with those estimated from independent-yield systematics, but are approximately 0.1 charge unit greater than predicted. Several partial isomer yields and isomer ratios were measured. These results provide additional information about the fractional production of isomeric states either directly from fission or from β decay. The absolute photon intensity for the 342-keV transition in the decay of Agg111 was measured to be 0.0668(±5%).

NUCLEAR REACTIONS, FISSION Pu240(n,f), E=14.8 MeV; measured fission yields, deduced fission mass distribution. Measured independent fission yields and partial isomeric yields. Agg111 measured Iγ.

  • Received 8 July 1977

DOI:https://doi.org/10.1103/PhysRevC.16.1907

©1977 American Physical Society

Authors & Affiliations

D. R. Nethaway and A. L. Prindle

  • University of California, Lawrence Livermore Laboratory, Livermore, California 94550

William A. Myers*, W. C. Fuqua, and M. V. Kantelo

  • McClellan Central Laboratory, 1155 Technical Operations Squadron, McClellan AFB, California 95652

  • *Present address: Lt. Col. William A. Myers, Defense Intelligence Agency, DT-1B, Washington, D. C. 20301.
  • Present address: Celanese Chemical Co. Technical Center, P. O. Box 9077, Corpus Christi, Texas 78408.

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Vol. 16, Iss. 5 — November 1977

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