Effects of pressure on the magnetic-structural and Griffiths-like transitions in Dy5Si3Ge

N. Marcano, P. A. Algarabel, J. Rodríguez Fernández, C. Magén, L. Morellón, Niraj K. Singh, K. A. Gschneidner, Jr., V. K. Pecharsky, and M. R. Ibarra
Phys. Rev. B 88, 214429 – Published 30 December 2013

Abstract

Magnetization studies have been performed on a polycrystalline sample of Dy5Si3Ge as a function of an applied magnetic field (up to 50 kOe) and hydrostatic pressure (up to 10 kbar) in the 5–300 K temperature range. The anomalous behavior of the magnetic susceptibility indicates that a Griffiths-like phase exists at low magnetic fields and pressures up to 10 kbar. We present evidence that the high-temperature second-order ferromagnetic transition can be coupled with the low-temperature first-order crystallographic transformation into a single first-order magnetic-crystallographic transformation using a magnetic field and hydrostatic pressure as tuning parameters. The effect of pressure on the Griffiths-like phase is reported and analyzed in the framework of the complex competition between the interslab and intraslab magnetic interactions.

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  • Received 3 June 2013
  • Revised 2 October 2013

DOI:https://doi.org/10.1103/PhysRevB.88.214429

©2013 American Physical Society

Authors & Affiliations

N. Marcano1,2,3, P. A. Algarabel2,3, J. Rodríguez Fernández4, C. Magén3,5,6, L. Morellón3,5, Niraj K. Singh7, K. A. Gschneidner, Jr.7,8, V. K. Pecharsky7, and M. R. Ibarra1,3,5

  • 1Centro Universitario de la Defensa, Academia General Militar Crta. Huesca s/n 50090 Zaragoza, Spain
  • 2Instituto de Ciencia de Materiales de Aragón, CSIC-Universidad de Zaragoza, 50009 Zaragoza, Spain
  • 3Departamento Física de la Materia Condensada, Universidad de Zaragoza, 50009 Zaragoza, Spain
  • 4Departamento CITIMAC, Universidad de Cantabria, 39005 Santander, Spain
  • 5Instituto de Nanociencia de Aragón, Universidad de Zaragoza, 50018 Zaragoza, Spain
  • 6Fundación ARAID, 50018 Zaragoza, Spain
  • 7Ames Laboratory, U.S. Department of Energy, Iowa State University, Ames, Iowa 50011-3020, USA
  • 8Department of Materials Science and Engineering, Iowa State University, Ames, Iowa, 50011-2030, USA

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Issue

Vol. 88, Iss. 21 — 1 December 2013

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