Abstract
We report high-magnetic-field thermal expansion and magnetostriction results on single crystals. Several phase transitions, both first and second order, are observed when the field is applied perpendicular to the crystallographic axis. The magnetic field dependence of the thermal-expansion coefficient above , where the magnetic correlations are negligible, can be explained supposing an almost pure ground state doublet, in apparent contradiction with neutron scattering experiments. Although the spin-lattice interaction is relevant in this compound, the effect of the magnetic correlations on the elastic properties is relatively weak, as revealed by resonant ultrasound spectroscopy experiments.
- Received 10 November 2004
DOI:https://doi.org/10.1103/PhysRevB.72.012407
©2005 American Physical Society