Electronic transport in quasi-one-dimensional arrays of gold nanocrystals

Klara Elteto, Xiao-Min Lin, and Heinrich M. Jaeger
Phys. Rev. B 71, 205412 – Published 26 May 2005

Abstract

We report on the fabrication and current-voltage (IV) characteristics of very narrow, striplike arrays of metal nanoparticles. The arrays were formed from gold nanocrystals self-assembled between in-plane electrodes. The local cross linking of the ligands by exposure to a focused electron beam and the subsequent removal of the unexposed regions produced arrays as narrow as four particles wide and sixty particles long, with a high degree of structural ordering. Remarkably, even for such quasi-one-dimensional strips, we found nonlinear, power-law IV characteristics similar to those of much wider two-dimensional (2D) arrays. However, in contrast to the robust behavior of the 2D arrays, the shape of the IV characteristics is much more sensitive to temperature changes and temperature cycling. Furthermore, at low temperatures we observed pronounced two-level current fluctuations indicative of discrete rearrangements in the current paths. We associate this behavior with the inherent high sensitivity of single-electron tunneling to the polarization caused by the quenched offset charges in the underlying substrate.

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  • Received 7 February 2005

DOI:https://doi.org/10.1103/PhysRevB.71.205412

©2005 American Physical Society

Authors & Affiliations

Klara Elteto1, Xiao-Min Lin2, and Heinrich M. Jaeger1

  • 1James Franck Institute and Department of Physics, University of Chicago, Chicago, Illinois 60637, USA
  • 2Materials Science Division, Chemistry Division and Center for Nanoscale Materials, Argonne National Laboratory, Argonne, Illinois 60439, USA

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Issue

Vol. 71, Iss. 20 — 15 May 2005

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