High-pressure phase of CeRu2: A magnetic superconductor with two charge states of Ru ions

A. V. Tsvyashchenko, L. N. Fomicheva, A. A. Sorokin, G. K. Ryasny, B. A. Komissarova, L. G. Shpinkova, K. V. Klementiev, A. V. Kuznetsov, A. P. Menushenkov, V. N. Trofimov, A. E. Primenko, and R. Cortes
Phys. Rev. B 65, 174513 – Published 22 April 2002
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Abstract

The intermetallic compounds LaRu2 and CeRu2, as well as several quasibinary systems Ce1xLaxRu2, were synthesized at a pressure of 8 GPa. The x-ray diffraction data showed the pure cubic C15 structure for all samples. The x-ray absorption measurements gave the value 3.23 for the Ce valence. Time-differential perturbed angular correlation measurements with the 111In-doped samples have shown (i) 111In substituted for Ru; (ii) in LaRu2 a single value of the quadrupole frequency νQ=234 MHz for the daughter 111Cd nuclei was observed; (iii) in CeRu2 two distinct equally populated sites for 111Cd were revealed with νQ=218 and νQ=153MHz. The low-temperature magnetic measurements showed that magnetic moments about 0.3μB per formula unit are inherent in all samples and indicated at a coexistence of superconductivity and magnetic ordering. In particular, the magnetic and superconducting correlations are developing, most probably, in the same system of ruthenium 4d electrons.

  • Received 15 August 2001

DOI:https://doi.org/10.1103/PhysRevB.65.174513

©2002 American Physical Society

Authors & Affiliations

A. V. Tsvyashchenko and L. N. Fomicheva

  • Vereshchagin Institute of High Pressure Physics, Russian Academy of Sciences, 142092 Troitsk, Moscow region, Russia

A. A. Sorokin, G. K. Ryasny, B. A. Komissarova, and L. G. Shpinkova

  • Skobeltsyn Institute of Nuclear Physics, Moscow State University, 119899 Moscow, Russia

K. V. Klementiev, A. V. Kuznetsov, and A. P. Menushenkov

  • Department of Quantum Electronics, Moscow Engineering Physics Institute, Kashirskoe shosse 31, 115409 Moscow, Russia

V. N. Trofimov

  • Joint Institute for Nuclear Research, Laboratory of Nuclear Problems, P.O. Box 79, Moscow, Russia

A. E. Primenko

  • Department of Low Temperature Physics, Moscow State University, 117234 Moscow, Russia

R. Cortes

  • Laboratoire pour l’ Utilisation du Rayonnement Electromagnetique, 91405, Orsay, France

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Vol. 65, Iss. 17 — 1 May 2002

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