Effect of interfacial states on the binding energies of electrons and holes in InAs/GaAs quantum dots

A. J. Williamson and Alex Zunger
Phys. Rev. B 58, 6724 – Published 15 September 1998
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Abstract

The interface between an InAs quantum dot and its GaAs cap in “self-assembled” nanostructures is nonhomogeneously strained. We show that this strain can lead to localization of a GaAs-derived X1c-type interfacial electron state. As hydrostatic pressure is applied, this state in the GaAs barrier turns into the conduction-band minimum of the InAs/GaAs dot system. Strain splits the degeneracy of this X1c state and is predicted to cause electrons to localize in the GaAs barrier above the pyramidal tip. Calculation (present work) or measurement (Itskevich et al.) of the emission energy from this state to the hole state can provide the hole binding energy, Δdot(h). Combining this with the zero-pressure electron-hole recombination energy gives the electron binding energy, Δdot(e). Our calculations show Δdot(h)270meV (weakly pressure dependent) and Δdot(e)100meV at P=0. The measured values are Δdot(h)235meV (weakly pressure dependent) and Δdot(e)50meV at P=0. We examine the discrepancy between these values in the light of wave-function localization and the pressure dependence of the hole binding energy.

  • Received 24 April 1998

DOI:https://doi.org/10.1103/PhysRevB.58.6724

©1998 American Physical Society

Authors & Affiliations

A. J. Williamson and Alex Zunger

  • National Renewable Energy Laboratory, Golden, Colorado 80401

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Vol. 58, Iss. 11 — 15 September 1998

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